A host-guest drug delivery nanosystem for supramolecular chemotherapy.

Calixarene Drug delivery Macrocyclic amphiphiles Molecular recognition Supramolecular chemotherapy

Journal

Journal of controlled release : official journal of the Controlled Release Society
ISSN: 1873-4995
Titre abrégé: J Control Release
Pays: Netherlands
ID NLM: 8607908

Informations de publication

Date de publication:
10 08 2020
Historique:
received: 11 12 2019
revised: 01 05 2020
accepted: 04 05 2020
pubmed: 21 5 2020
medline: 22 6 2021
entrez: 21 5 2020
Statut: ppublish

Résumé

Supramolecular chemotherapy is currently a new strategy to improve the therapeutic efficacy as well as overcome the side effects of traditional chemotherapy. Herein, a supramolecular chemotherapy platform based on the pegylated guanidinium-modified calix[5]arene pentadodecyl ether (GC5A-12C) nanoassembly was prepared. Three commercially available antitumor drugs: oxaliplatin, methotrexate and chlorambucil, all showed strong binding to this GC5A-12C nanocarrier. The supramolecular nanodrugs achieved higher anticancer performances compared with free drugs in cell experiments. Furthermore, the cellular uptake mechanisms and efficacy are confirmed by fluorescence imaging.

Identifiants

pubmed: 32430277
pii: S0168-3659(20)30283-2
doi: 10.1016/j.jconrel.2020.05.008
pii:
doi:

Substances chimiques

Antineoplastic Agents 0
Pharmaceutical Preparations 0
Oxaliplatin 04ZR38536J
Methotrexate YL5FZ2Y5U1

Types de publication

Journal Article Research Support, Non-U.S. Gov't

Langues

eng

Sous-ensembles de citation

IM

Pagination

124-133

Informations de copyright

Copyright © 2020 Elsevier B.V. All rights reserved.

Auteurs

Xin-Yue Hu (XY)

College of Chemistry, Key Laboratory of Functional Polymer Materials (Ministry of Education), State Key Laboratory of Elemento-Organic Chemistry, Nankai University, Tianjin 300071, PR China.

Jie Gao (J)

College of Chemistry, Key Laboratory of Functional Polymer Materials (Ministry of Education), State Key Laboratory of Elemento-Organic Chemistry, Nankai University, Tianjin 300071, PR China.

Fang-Yuan Chen (FY)

College of Chemistry, Key Laboratory of Functional Polymer Materials (Ministry of Education), State Key Laboratory of Elemento-Organic Chemistry, Nankai University, Tianjin 300071, PR China.

Dong-Sheng Guo (DS)

College of Chemistry, Key Laboratory of Functional Polymer Materials (Ministry of Education), State Key Laboratory of Elemento-Organic Chemistry, Nankai University, Tianjin 300071, PR China. Electronic address: dshguo@nankai.edu.cn.

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Classifications MeSH