Control of zeolite pore interior for chemoselective alkyne/olefin separations.


Journal

Science (New York, N.Y.)
ISSN: 1095-9203
Titre abrégé: Science
Pays: United States
ID NLM: 0404511

Informations de publication

Date de publication:
29 05 2020
Historique:
received: 23 07 2019
revised: 16 01 2020
accepted: 10 04 2020
entrez: 30 5 2020
pubmed: 30 5 2020
medline: 30 5 2020
Statut: ppublish

Résumé

The efficient removal of alkyne impurities for the production of polymer-grade lower olefins remains an important and challenging goal for many industries. We report a strategy to control the pore interior of faujasite (FAU) zeolites by the confinement of isolated open nickel(II) sites in their six-membered rings. Under ambient conditions, Ni@FAU showed remarkable adsorption of alkynes and efficient separations of acetylene/ethylene, propyne/propylene, and butyne/1,3-butadiene mixtures, with unprecedented dynamic separation selectivities of 100, 92, and 83, respectively. In situ neutron diffraction and inelastic neutron scattering revealed that confined nickel(II) sites enabled chemoselective and reversible binding to acetylene through the formation of metastable [Ni(II)(C

Identifiants

pubmed: 32467390
pii: 368/6494/1002
doi: 10.1126/science.aay8447
doi:

Types de publication

Journal Article Research Support, Non-U.S. Gov't Research Support, U.S. Gov't, Non-P.H.S.

Langues

eng

Sous-ensembles de citation

IM

Pagination

1002-1006

Informations de copyright

Copyright © 2020 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works.

Auteurs

Yuchao Chai (Y)

School of Materials Science and Engineering and National Institute for Advanced Materials, Nankai University, Tianjin 300350, China.

Xue Han (X)

Department of Chemistry, The University of Manchester, Manchester, M13 9PL, UK.

Weiyao Li (W)

Department of Chemistry, The University of Manchester, Manchester, M13 9PL, UK.

Shanshan Liu (S)

School of Materials Science and Engineering and National Institute for Advanced Materials, Nankai University, Tianjin 300350, China.

Sikai Yao (S)

School of Materials Science and Engineering and National Institute for Advanced Materials, Nankai University, Tianjin 300350, China.

Chong Wang (C)

State Key Laboratory of Molecular Reaction Dynamics, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian 116023, China.

Wei Shi (W)

Key Laboratory of Advanced Energy Materials Chemistry of Ministry of Education, Nankai University, Tianjin 300071, China.

Ivan da-Silva (I)

ISIS Facility, Science and Technology Facilities Council (STFC), Rutherford Appleton Laboratory, Chilton, Oxfordshire, OX11 0QX, UK.

Pascal Manuel (P)

ISIS Facility, Science and Technology Facilities Council (STFC), Rutherford Appleton Laboratory, Chilton, Oxfordshire, OX11 0QX, UK.

Yongqiang Cheng (Y)

Neutron Scattering Division, Neutron Sciences Directorate, Oak Ridge National Laboratory (ORNL), Oak Ridge, TN 37831, USA.

Luke D Daemen (LD)

Neutron Scattering Division, Neutron Sciences Directorate, Oak Ridge National Laboratory (ORNL), Oak Ridge, TN 37831, USA.

Anibal J Ramirez-Cuesta (AJ)

Neutron Scattering Division, Neutron Sciences Directorate, Oak Ridge National Laboratory (ORNL), Oak Ridge, TN 37831, USA.

Chiu C Tang (CC)

Diamond Light Source, Harwell Science and Innovation Campus, Didcot, Oxfordshire, OX11 0DE, UK.

Ling Jiang (L)

State Key Laboratory of Molecular Reaction Dynamics, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian 116023, China.

Sihai Yang (S)

Department of Chemistry, The University of Manchester, Manchester, M13 9PL, UK. sihai.yang@manchester.ac.uk lild@nankai.edu.cn.

Naijia Guan (N)

School of Materials Science and Engineering and National Institute for Advanced Materials, Nankai University, Tianjin 300350, China.
Key Laboratory of Advanced Energy Materials Chemistry of Ministry of Education, Nankai University, Tianjin 300071, China.

Landong Li (L)

School of Materials Science and Engineering and National Institute for Advanced Materials, Nankai University, Tianjin 300350, China. sihai.yang@manchester.ac.uk lild@nankai.edu.cn.
Key Laboratory of Advanced Energy Materials Chemistry of Ministry of Education, Nankai University, Tianjin 300071, China.

Classifications MeSH