Synthesis, characterization and oxygen sensitivity of cyclophosphazene equipped-iridium (III) complexes.

Cyclophosphazenes Electrospun mats Iridium (III) complexes Oxygen sensitivity Phosphorescence

Journal

Spectrochimica acta. Part A, Molecular and biomolecular spectroscopy
ISSN: 1873-3557
Titre abrégé: Spectrochim Acta A Mol Biomol Spectrosc
Pays: England
ID NLM: 9602533

Informations de publication

Date de publication:
05 Oct 2020
Historique:
received: 16 01 2020
revised: 21 04 2020
accepted: 13 05 2020
pubmed: 6 6 2020
medline: 6 6 2020
entrez: 6 6 2020
Statut: ppublish

Résumé

In this work, synthesis, characterization and oxygen sensing abilities of the cyclophosphazene-free and phenyl and naphtoxy-substituted cyclophosphazene bearing iridium (III) complexes (Ir-I, Ir-II and Ir-III) were presented. The complexes were characterized by NMR, absorption and emission spectroscopies, luminescence lifetime and quantum yield measurements. The molecules were successfully embedded in the ethyl cellulose matrix to fabricate the oxygen sensing electrospun mats via electrospinning technique. Oxygen induced luminescence of the iridium complexes around 600 nm has been followed as the analytical signal during oxygen sensitivity studies. They exhibited blue shifted, quenched emission towards triplet oxygen. The napthoxy substituted derivative exhibited 2.70 fold enhanced I

Identifiants

pubmed: 32502815
pii: S1386-1425(20)30469-8
doi: 10.1016/j.saa.2020.118490
pii:
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

118490

Informations de copyright

Copyright © 2020 Elsevier B.V. All rights reserved.

Déclaration de conflit d'intérêts

Declaration of competing interest The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper.

Auteurs

Merve Zeyrek Ongun (M)

Dokuz Eylul University, Chemistry Technology Program, Izmir Vocational High School, 35360 Izmir, Turkey.

Murat Sahin (M)

Gebze Technical University, Faculty of Science, Department of Chemistry, 41400 Gebze, Kocaeli, Turkey.

Tugce Akbal (T)

Gebze Technical University, Faculty of Science, Department of Chemistry, 41400 Gebze, Kocaeli, Turkey.

Neslihan Avsar (N)

Gebze Technical University, Faculty of Science, Department of Chemistry, 41400 Gebze, Kocaeli, Turkey.

Hayriye Karakas (H)

Gebze Technical University, Faculty of Science, Department of Chemistry, 41400 Gebze, Kocaeli, Turkey.

Kadriye Ertekin (K)

Dokuz Eylul University, Faculty of Sciences, Department of Chemistry, 35160 Buca, Izmir, Turkey.

Devrim Atilla (D)

Gebze Technical University, Faculty of Science, Department of Chemistry, 41400 Gebze, Kocaeli, Turkey.

Hanife İbişoğlu (H)

Gebze Technical University, Faculty of Science, Department of Chemistry, 41400 Gebze, Kocaeli, Turkey. Electronic address: ibisoglu@gtu.edu.tr.

Sevinc Zehra Topal (SZ)

Gebze Technical University, Faculty of Science, Department of Chemistry, 41400 Gebze, Kocaeli, Turkey. Electronic address: sztopal@gtu.edu.tr.

Classifications MeSH