Synthesis, admetSAR Predictions, DPPH Radical Scavenging Activity, and Potent Anti-mycobacterial Studies of Hydrazones of Substituted 4-(anilino methyl) benzohydrazides (Part 2).


Journal

Current computer-aided drug design
ISSN: 1875-6697
Titre abrégé: Curr Comput Aided Drug Des
Pays: United Arab Emirates
ID NLM: 101265750

Informations de publication

Date de publication:
2021
Historique:
received: 11 01 2020
revised: 16 04 2020
accepted: 20 05 2020
pubmed: 17 6 2020
medline: 14 1 2022
entrez: 16 6 2020
Statut: ppublish

Résumé

For the past several decades, the presence of tuberculosis (TB) is being remarked as the most common infectious disease leading to mortality. Hydrazone containing azometine group (-NHN=CH-) compounds have been reported for a broad range of bioactivities such as antiplatelet, analgesic, anti-inflammatory, anticonvulsant, antidepressant, antimalarial, vasodilator, antiviral, and antimicrobial, etc. Methods: For the synthesis of compounds (4a-4d) and (6a-6e), aromatic amines were treated with methyl terephthalaldehydate in methanol, giving Schiff's bases, followed by reductive amination and further treatment with hydrazine hydrate gave acid hydrazides (4a-4d). These acid hydrazides were then treated with different aromatic aldehydes to yield hydrazones (6a-6d). All the synthesized compounds were subjected to FT-IR, NMR, and UV spectroscopic characterization. Compounds (4a-4d) and (6a-6e) were found to have highly potent activity against Mycobacteria tuberculosis (Vaccine strain, H37 RV strains): ATCC No- 27294 (MIC:1.6-6.25 μg/mL) than standard anti-TB drugs. The compounds exhibited good radical scavenging potentials(0- 69.2%), as checked from DPPH protocol. All compounds also demonstrated good in-silico ADMET results. The current study revealed promising in vitro anti-tuberculosis and anti-oxidant profiles of hydrazide-hydrazone analogues.

Sections du résumé

BACKGROUND BACKGROUND
For the past several decades, the presence of tuberculosis (TB) is being remarked as the most common infectious disease leading to mortality.
OBJECTIVE OBJECTIVE
Hydrazone containing azometine group (-NHN=CH-) compounds have been reported for a broad range of bioactivities such as antiplatelet, analgesic, anti-inflammatory, anticonvulsant, antidepressant, antimalarial, vasodilator, antiviral, and antimicrobial, etc. Methods: For the synthesis of compounds (4a-4d) and (6a-6e), aromatic amines were treated with methyl terephthalaldehydate in methanol, giving Schiff's bases, followed by reductive amination and further treatment with hydrazine hydrate gave acid hydrazides (4a-4d). These acid hydrazides were then treated with different aromatic aldehydes to yield hydrazones (6a-6d). All the synthesized compounds were subjected to FT-IR, NMR, and UV spectroscopic characterization.
RESULTS RESULTS
Compounds (4a-4d) and (6a-6e) were found to have highly potent activity against Mycobacteria tuberculosis (Vaccine strain, H37 RV strains): ATCC No- 27294 (MIC:1.6-6.25 μg/mL) than standard anti-TB drugs. The compounds exhibited good radical scavenging potentials(0- 69.2%), as checked from DPPH protocol. All compounds also demonstrated good in-silico ADMET results.
CONCLUSION CONCLUSIONS
The current study revealed promising in vitro anti-tuberculosis and anti-oxidant profiles of hydrazide-hydrazone analogues.

Identifiants

pubmed: 32538732
pii: CAD-EPUB-107360
doi: 10.2174/1573409916666200615141047
doi:

Substances chimiques

Antitubercular Agents 0
Hydrazones 0

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

493-503

Informations de copyright

Copyright© Bentham Science Publishers; For any queries, please email at epub@benthamscience.net.

Auteurs

Vijay J Desale (VJ)

Department of Chemistry, Government of Maharashtra's Ismail Yusuf College, Jogeshwari, Mumbai-400060, India.

Suraj N Mali (SN)

Government College of Pharmacy, Karad, Maharashtra, India.

Bapu R Thorat (BR)

Department of Chemistry, Government of Maharashtra's Ismail Yusuf College, Jogeshwari, Mumbai-400060, India.

Ramesh S Yamgar (RS)

Department of Chemistry, Patkar-Varde College of Arts, Science and Commerce, Goregaon (W), Mumbai 400 062, India.

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Classifications MeSH