Measuring and modelling mechanochemical reaction kinetics.


Journal

Chemical communications (Cambridge, England)
ISSN: 1364-548X
Titre abrégé: Chem Commun (Camb)
Pays: England
ID NLM: 9610838

Informations de publication

Date de publication:
14 Jul 2020
Historique:
pubmed: 20 6 2020
medline: 20 6 2020
entrez: 20 6 2020
Statut: ppublish

Résumé

Quasi-static density functional theory calculations of the rate of mechanochemical decomposition of methyl thiolate species adsorbed on Cu(100) accurately reproduce the experimental normal-stress dependent rates measured in ultrahigh vacuum by an atomic force microscopy tip. This allows precise analytical models for mechanochemical reaction kinetics to be developed.

Identifiants

pubmed: 32558870
doi: 10.1039/d0cc02992k
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

7730-7733

Auteurs

Alejandro Boscoboinik (A)

Department of Chemistry and Biochemistry and Laboratory for Surface Studies University of Wisconsin-Milwaukee, Milwaukee, WI 53211, USA. wtt@uwm.edu.

Dustin Olson (D)

Department of Chemistry and Biochemistry and Laboratory for Surface Studies University of Wisconsin-Milwaukee, Milwaukee, WI 53211, USA. wtt@uwm.edu.

Heather Adams (H)

Department of Chemistry and Biochemistry and Laboratory for Surface Studies University of Wisconsin-Milwaukee, Milwaukee, WI 53211, USA. wtt@uwm.edu.

Nicholas Hopper (N)

Department of Chemistry and Biochemistry and Laboratory for Surface Studies University of Wisconsin-Milwaukee, Milwaukee, WI 53211, USA. wtt@uwm.edu.

Wilfred T Tysoe (WT)

Department of Chemistry and Biochemistry and Laboratory for Surface Studies University of Wisconsin-Milwaukee, Milwaukee, WI 53211, USA. wtt@uwm.edu.

Classifications MeSH