High-Performance and Reliable Lead-Free Layered-Perovskite Transistors.
complementary inverters
grain size engineering
lead-free perovskite transistors
self-passivation
solution processing
Journal
Advanced materials (Deerfield Beach, Fla.)
ISSN: 1521-4095
Titre abrégé: Adv Mater
Pays: Germany
ID NLM: 9885358
Informations de publication
Date de publication:
Aug 2020
Aug 2020
Historique:
received:
21
04
2020
revised:
13
06
2020
pubmed:
26
6
2020
medline:
26
6
2020
entrez:
26
6
2020
Statut:
ppublish
Résumé
Perovskites have been intensively investigated for their use in solar cells and light-emitting diodes. However, research on their applications in thin-film transistors (TFTs) has drawn less attention despite their high intrinsic charge carrier mobility. In this study, the universal approaches for high-performance and reliable p-channel lead-free phenethylammonium tin iodide TFTs are reported. These include self-passivation for grain boundary by excess phenethylammonium iodide, grain crystallization control by adduct, and iodide vacancy passivation through oxygen treatment. It is found that the grain boundary passivation can increase TFT reproducibility and reliability, and the grain size enlargement can hike the TFT performance, thus, enabling the first perovskite-based complementary inverter demonstration with n-channel indium gallium zinc oxide TFTs. The inverter exhibits a high gain over 30 with an excellent noise margin. This work aims to provide widely applicable and repeatable methods to make the gate more open for intensive efforts toward high-performance printed perovskite TFTs.
Identifiants
pubmed: 32584475
doi: 10.1002/adma.202002717
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
e2002717Subventions
Organisme : Ministry of Science & ICT
Organisme : NRF
Organisme : Korean government
ID : 2017R1E1A1A01075360
Organisme : Korean government
ID : NRF-2018R1A2B2002875
Organisme : Centre for Advanced Soft-Electronics
ID : 2013M3A6A5073183
Informations de copyright
© 2020 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
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