Poly(siloxane imide) Binder for Silicon-Based Lithium-Ion Battery Anodes via Rigidness/Softness Coupling.
Binder
Lithium-ion batteries
Poly(siloxane imide)
Polyimide
Silicon anodes
Journal
Chemistry, an Asian journal
ISSN: 1861-471X
Titre abrégé: Chem Asian J
Pays: Germany
ID NLM: 101294643
Informations de publication
Date de publication:
01 Sep 2020
01 Sep 2020
Historique:
received:
25
05
2020
pubmed:
2
7
2020
medline:
2
7
2020
entrez:
2
7
2020
Statut:
ppublish
Résumé
Binders play a crucial role in maintaining mechanical integrity of electrodes in lithium-ion batteries. However, the conventional binders lack proper elasticity, and they are not suitable for high-performance silicon anodes featuring huge volume change during cycling. Herein, a poly(siloxane imide) copolymer (PSI) has been designed, synthesized, and utilized as a binder for silicon-based anodes. A rigidness/softness coupling mechanism is demonstrated by the PSI binder, which can accommodate volume expansion of the silicon anode upon lithiation. The electrochemical performance in terms of cyclic stability and rate capability can be effectively improved with the PSI binder as demonstrated by a silicon nanoparticle anode.
Identifiants
pubmed: 32608136
doi: 10.1002/asia.202000633
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
2674-2680Subventions
Organisme : National Key R&D Program of China
ID : 2016YFB0100100
Organisme : National Natural Science Foundation of China
ID : 51702335
Organisme : National Natural Science Foundation of China
ID : 21773279
Organisme : Zhejiang Non-profit Technology Applied Research Program
ID : LGG19B010001
Organisme : Ningbo Municipal Natural Science Foundation
ID : 2018 A610084
Organisme : CAS-EU S&T cooperation partner program
ID : 174433KYSB20150013
Organisme : Key Laboratory of Bio-based Polymeric Materials of Zhejiang Province
Organisme : European Union's Horizon 2020 research and innovation programme under the Marie Sklodowska-Curie grant agreement
ID : 655881
Informations de copyright
© 2020 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim.
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