Hybrid Photo- and Thermal Catalyst System for Continuous CO

CO2 conversion light absorption photocatalysis photocatalytic film photoreactor photothermal reverse water gas shift (RWGS) reaction solar fuel

Journal

ACS applied materials & interfaces
ISSN: 1944-8252
Titre abrégé: ACS Appl Mater Interfaces
Pays: United States
ID NLM: 101504991

Informations de publication

Date de publication:
29 Jul 2020
Historique:
pubmed: 2 7 2020
medline: 2 7 2020
entrez: 2 7 2020
Statut: ppublish

Résumé

Heterogeneous thermal catalytic processes are vital for industrial production of fuels, fertilizers, and other chemicals necessary for sustaining human life. However, these processes are highly energy-intensive, requiring a vast consumption of fossil fuels. An emerging class of heterogeneous catalysts that are thermally driven but also exhibit a photochemically enhanced rate can potentially reduce process energy intensity by partially substituting conventional heat (where fossil fuels are needed) with solar energy. Such catalyst systems have yet to be practically utilized. Here, we demonstrate a compact electrically heated photo- and thermal annular reactor module to reduce CO

Identifiants

pubmed: 32609486
doi: 10.1021/acsami.0c06232
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

33613-33620

Auteurs

Abhinav Mohan (A)

Department of Mechanical and Industrial Engineering, University of Toronto, 5 King's College Rd, Toronto, ON M5S 3G8, Canada.

Ulrich Ulmer (U)

Department of Chemistry, University of Toronto, 80 Saint George Street, Toronto, ON M5S 3H6, Canada.

Lourdes Hurtado (L)

Department of Chemistry, University of Toronto, 80 Saint George Street, Toronto, ON M5S 3H6, Canada.

Joel Loh (J)

Department of Electrical & Computer Engineering, University of Toronto, 10 King's College Road, Toronto, ON M5S 3G4, Canada.

Young Feng Li (YF)

Department of Chemistry, University of Toronto, 80 Saint George Street, Toronto, ON M5S 3H6, Canada.

Athanasios A Tountas (AA)

Department of Chemical Engineering and Applied Chemistry, University of Toronto, 200 College Street, Toronto, ON M5S 3E5, Canada.

Carola Krevert (C)

Department of Chemistry, University of Toronto, 80 Saint George Street, Toronto, ON M5S 3H6, Canada.

Chakyu Chan (C)

Department of Chemistry, University of Toronto, 80 Saint George Street, Toronto, ON M5S 3H6, Canada.

Yilei Liang (Y)

Department of Chemical Engineering and Applied Chemistry, University of Toronto, 200 College Street, Toronto, ON M5S 3E5, Canada.

Peter Brodersen (P)

Department of Chemical Engineering and Applied Chemistry, University of Toronto, 200 College Street, Toronto, ON M5S 3E5, Canada.

Mohini M Sain (MM)

Department of Mechanical and Industrial Engineering, University of Toronto, 5 King's College Rd, Toronto, ON M5S 3G8, Canada.

Geoffrey A Ozin (GA)

Department of Chemistry, University of Toronto, 80 Saint George Street, Toronto, ON M5S 3H6, Canada.

Classifications MeSH