Revealing Nanoscale Chemical Heterogeneities in Polycrystalline Mo-BiVO

bismuth vanadate chemical heterogeneity first principles scanning X-ray microscopy water splitting

Journal

Small (Weinheim an der Bergstrasse, Germany)
ISSN: 1613-6829
Titre abrégé: Small
Pays: Germany
ID NLM: 101235338

Informations de publication

Date de publication:
Sep 2020
Historique:
received: 10 03 2020
revised: 04 06 2020
pubmed: 6 8 2020
medline: 6 8 2020
entrez: 6 8 2020
Statut: ppublish

Résumé

The activity of polycrystalline thin film photoelectrodes is impacted by local variations of the material properties due to the exposure of different crystal facets and the presence of grain/domain boundaries. Here a multi-modal approach is applied to correlate nanoscale heterogeneities in chemical composition and electronic structure with nanoscale morphology in polycrystalline Mo-BiVO

Identifiants

pubmed: 32755006
doi: 10.1002/smll.202001600
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

e2001600

Subventions

Organisme : U.S. Department of Energy
ID : DE-AC02-05CH11231
Organisme : U.S. Department of Energy
ID : DE-SC0004993
Organisme : DGI-UNAB Regular
ID : DI-21-18/"REG"
Organisme : FONDECYT
ID : 11180590
Organisme : DFG
ID : EXC 2089/1
Organisme : DFG
ID : 390776260

Informations de copyright

© 2020 The Authors. Published by Wiley-VCH GmbH.

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Auteurs

Johanna Eichhorn (J)

Chemical Sciences Division and Joint Center for Artificial Photosynthesis, Lawrence Berkeley National Laboratory, 1 Cyclotron Road, Berkeley, CA, 94720, USA.
Walter Schottky Institut and Physik Department, Technische Universität München, Am Coulombwall 4, Garching, 85748, Germany.

Sebastian E Reyes-Lillo (SE)

Departamento de Ciencias Físicas, Universidad Andres Bello, Santiago, 837-0136, Chile.

Subhayan Roychoudhury (S)

Advanced Light Source, Lawrence Berkeley National Laboratory, Berkeley, CA, 94720, USA.
The Molecular Foundry, Lawrence Berkeley National Laboratory, Berkeley, CA, 94720, USA.

Shawn Sallis (S)

Advanced Light Source, Lawrence Berkeley National Laboratory, Berkeley, CA, 94720, USA.

Johannes Weis (J)

Chemical Sciences Division and Joint Center for Artificial Photosynthesis, Lawrence Berkeley National Laboratory, 1 Cyclotron Road, Berkeley, CA, 94720, USA.

David M Larson (DM)

Chemical Sciences Division and Joint Center for Artificial Photosynthesis, Lawrence Berkeley National Laboratory, 1 Cyclotron Road, Berkeley, CA, 94720, USA.

Jason K Cooper (JK)

Chemical Sciences Division and Joint Center for Artificial Photosynthesis, Lawrence Berkeley National Laboratory, 1 Cyclotron Road, Berkeley, CA, 94720, USA.

Ian D Sharp (ID)

Chemical Sciences Division and Joint Center for Artificial Photosynthesis, Lawrence Berkeley National Laboratory, 1 Cyclotron Road, Berkeley, CA, 94720, USA.
Walter Schottky Institut and Physik Department, Technische Universität München, Am Coulombwall 4, Garching, 85748, Germany.

David Prendergast (D)

The Molecular Foundry, Lawrence Berkeley National Laboratory, Berkeley, CA, 94720, USA.

Francesca M Toma (FM)

Chemical Sciences Division and Joint Center for Artificial Photosynthesis, Lawrence Berkeley National Laboratory, 1 Cyclotron Road, Berkeley, CA, 94720, USA.

Classifications MeSH