Linear Coordination Polymer Synthesis from Bis-Catechol Functionalized RAFT Polymers.
RAFT
catechol
coordination polymer
Journal
Macromolecular rapid communications
ISSN: 1521-3927
Titre abrégé: Macromol Rapid Commun
Pays: Germany
ID NLM: 9888239
Informations de publication
Date de publication:
Sep 2020
Sep 2020
Historique:
received:
09
07
2020
revised:
20
07
2020
pubmed:
7
8
2020
medline:
22
6
2021
entrez:
7
8
2020
Statut:
ppublish
Résumé
Catechol-Fe(III) complexes contain some of the strongest known metal-chelate coordination bonds. Despite this, they have until now not been utilized in (polymeric linker) linear coordination polymer (LCP) synthesis. With the view of generating catechol end-functional polymers, a new, symmetrical bis-catechol functionalized trithiocarbonate reversible addition fragmentation chain transfer (RAFT) agent is synthesized (CatDMAT). Acrylamide (AM) and dimethylacrylamide (DMA) polymerizations are conducted with CatDMAT using direct photoactivation RAFT polymerization to yield bis-catechol end-functionalized homo- and block-copolymers of molecular weight 10-15 kDa. Catechol-Fe(III) LCPs are successfully formed from the telechelic catechol polymers by bis-complexation to Fe(III). The tetrahedral bis-complex is detected by UV-vis spectroscopy (λ
Identifiants
pubmed: 32757259
doi: 10.1002/marc.202000366
doi:
Substances chimiques
Catechols
0
Ferric Compounds
0
Polymers
0
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
e2000366Subventions
Organisme : Chemicals and Plastics Manufacturing Innovation Network and Training Program at Monash University
Informations de copyright
© 2020 Wiley-VCH GmbH.
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