Quantum Device Emulates the Dynamics of Two Coupled Oscillators.


Journal

The journal of physical chemistry letters
ISSN: 1948-7185
Titre abrégé: J Phys Chem Lett
Pays: United States
ID NLM: 101526034

Informations de publication

Date de publication:
03 Sep 2020
Historique:
pubmed: 14 8 2020
medline: 14 8 2020
entrez: 14 8 2020
Statut: ppublish

Résumé

Our quantum device is a solid-state array of semiconducting quantum dots that is addressed and read by 2D electronic spectroscopy. The experimental ultrafast dynamics of the device is well simulated by solving the time-dependent Schrödinger equation for a Hamiltonian that describes the lower electronically excited states of the dots and three laser pulses. The time evolution induced in the electronic states of the quantum device is used to emulate the quite different nonequilibrium vibrational dynamics of a linear triatomic molecule. We simulate the energy transfer between the two local oscillators and, in a more elaborate application, the expectation values of the quantum mechanical creation and annihilation operators of each local oscillator. The simulation uses the electronic coherences engineered in the device upon interaction with a specific sequence of ultrafast pulses. The algorithm uses the algebraic description of the dynamics of the physical problem and of the hardware.

Identifiants

pubmed: 32787197
doi: 10.1021/acs.jpclett.0c01880
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

6990-6995

Auteurs

Ksenia Komarova (K)

The Fritz Haber Center for Molecular Dynamics and Institute of Chemistry, The Hebrew University of Jerusalem, Jerusalem 91904, Israel.

Hugo Gattuso (H)

Theoretical Physical Chemistry, UR MolSys B6c, University of Liège, B4000 Liège, Belgium.

R D Levine (RD)

The Fritz Haber Center for Molecular Dynamics and Institute of Chemistry, The Hebrew University of Jerusalem, Jerusalem 91904, Israel.

F Remacle (F)

The Fritz Haber Center for Molecular Dynamics and Institute of Chemistry, The Hebrew University of Jerusalem, Jerusalem 91904, Israel.
Theoretical Physical Chemistry, UR MolSys B6c, University of Liège, B4000 Liège, Belgium.

Classifications MeSH