Photothermogenetic inhibition of cancer stemness by near-infrared-light-activatable nanocomplexes.


Journal

Nature communications
ISSN: 2041-1723
Titre abrégé: Nat Commun
Pays: England
ID NLM: 101528555

Informations de publication

Date de publication:
17 08 2020
Historique:
received: 10 09 2019
accepted: 17 07 2020
entrez: 19 8 2020
pubmed: 19 8 2020
medline: 9 9 2020
Statut: epublish

Résumé

Strategies for eradicating cancer stem cells (CSCs) are urgently required because CSCs are resistant to anticancer drugs and cause treatment failure, relapse and metastasis. Here, we show that photoactive functional nanocarbon complexes exhibit unique characteristics, such as homogeneous particle morphology, high water dispersibility, powerful photothermal conversion, rapid photoresponsivity and excellent photothermal stability. In addition, the present biologically permeable second near-infrared (NIR-II) light-induced nanocomplexes photo-thermally trigger calcium influx into target cells overexpressing the transient receptor potential vanilloid family type 2 (TRPV2). This combination of nanomaterial design and genetic engineering effectively eliminates cancer cells and suppresses stemness of cancer cells in vitro and in vivo. Finally, in molecular analyses of mechanisms, we show that inhibition of cancer stemness involves calcium-mediated dysregulation of the Wnt/β-catenin signalling pathway. The present technological concept may lead to innovative therapies to address the global issue of refractory cancers.

Identifiants

pubmed: 32807785
doi: 10.1038/s41467-020-17768-3
pii: 10.1038/s41467-020-17768-3
pmc: PMC7431860
doi:

Substances chimiques

Calcium Channels 0
TRPV Cation Channels 0
Trpv2 protein, mouse 0
Calcium SY7Q814VUP

Types de publication

Journal Article Research Support, Non-U.S. Gov't

Langues

eng

Sous-ensembles de citation

IM

Pagination

4117

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Auteurs

Yue Yu (Y)

Graduate School of Advanced Science and Technology, Japan Advanced Institute of Science and Technology, 1-1 Asahidai, Nomi, Ishikawa, 923-1292, Japan.
Biomedical Research Institute, National Institute of Advanced Industrial Science & Technology (AIST), Ikeda, 563-8577, Japan.

Xi Yang (X)

Graduate School of Advanced Science and Technology, Japan Advanced Institute of Science and Technology, 1-1 Asahidai, Nomi, Ishikawa, 923-1292, Japan.

Sheethal Reghu (S)

Graduate School of Advanced Science and Technology, Japan Advanced Institute of Science and Technology, 1-1 Asahidai, Nomi, Ishikawa, 923-1292, Japan.

Sunil C Kaul (SC)

AIST-INDIA DAILAB, DBT-AIST International Center for Translational & Environmental Research (DAICENTER), Cellular and Molecular Biotechnology Research Institute, AIST, Tsukuba, 305-8565, Japan.

Renu Wadhwa (R)

AIST-INDIA DAILAB, DBT-AIST International Center for Translational & Environmental Research (DAICENTER), Cellular and Molecular Biotechnology Research Institute, AIST, Tsukuba, 305-8565, Japan.

Eijiro Miyako (E)

Graduate School of Advanced Science and Technology, Japan Advanced Institute of Science and Technology, 1-1 Asahidai, Nomi, Ishikawa, 923-1292, Japan. e-miyako@jaist.ac.jp.

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