Adduct of the blistering warfare agent sesquimustard with human serum albumin and its mass spectrometric identification for biomedical verification of exposure.


Journal

Analytical and bioanalytical chemistry
ISSN: 1618-2650
Titre abrégé: Anal Bioanal Chem
Pays: Germany
ID NLM: 101134327

Informations de publication

Date de publication:
Nov 2020
Historique:
received: 10 07 2020
accepted: 25 08 2020
revised: 07 08 2020
pubmed: 10 9 2020
medline: 21 5 2021
entrez: 9 9 2020
Statut: ppublish

Résumé

Apart from the well-known sulfur mustard (SM), additional sulfur-containing blistering chemical warfare agents exist. Sesquimustard (Q) is one of them and five times more blistering than SM. It is a common impurity in mustard mixtures and regularly found in old munitions but can also be used in pure form. Compared to the extensive literature on SM, very little experimental data is available on Q and no protein biomarkers of exposure have been reported. We herein report for the first time the adduct of Q with the nucleophilic Cys

Identifiants

pubmed: 32902690
doi: 10.1007/s00216-020-02917-w
pii: 10.1007/s00216-020-02917-w
pmc: PMC7550388
doi:

Substances chimiques

Biomarkers 0
Chemical Warfare Agents 0
Mustard Compounds 0
Serum Albumin, Human ZIF514RVZR

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

7723-7737

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Auteurs

Marc-Michael Blum (MM)

Blum - Scientific Services, Björnsonweg 70d, 22587, Hamburg, Germany.

Annika Richter (A)

Department of Chemistry, Humboldt-Universität zu Berlin, Brook-Taylor-Straße 2, 12489, Berlin, Germany.

Markus Siegert (M)

Department of Chemistry, Humboldt-Universität zu Berlin, Brook-Taylor-Straße 2, 12489, Berlin, Germany.
Bundeswehr Institute of Pharmacology and Toxicology, Neuherbergstraße 11, 80937, Munich, Germany.

Horst Thiermann (H)

Bundeswehr Institute of Pharmacology and Toxicology, Neuherbergstraße 11, 80937, Munich, Germany.

Harald John (H)

Bundeswehr Institute of Pharmacology and Toxicology, Neuherbergstraße 11, 80937, Munich, Germany. haraldjohn@bundeswehr.org.

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Classifications MeSH