Universal Low-Frequency Vibrational Modes in Silica Glasses.


Journal

Physical review letters
ISSN: 1079-7114
Titre abrégé: Phys Rev Lett
Pays: United States
ID NLM: 0401141

Informations de publication

Date de publication:
21 Aug 2020
Historique:
received: 12 03 2020
revised: 09 07 2020
accepted: 21 07 2020
entrez: 10 9 2020
pubmed: 11 9 2020
medline: 11 9 2020
Statut: ppublish

Résumé

It was recently shown that different simple models of glass formers with binary interactions define a universality class in terms of the density of states of their quasilocalized low-frequency modes. Explicitly, once the hybridization with standard Debye (extended) modes is avoided, a number of such models exhibit a universal density of states, depending on the mode frequencies as D(ω)∼ω^{4}. It is unknown, however, how wide this universality class is, and whether it also pertains to more realistic models of glass formers. To address this issue we present analysis of the quasilocalized modes in silica, a network glass that has both binary and ternary interactions. We conclude that in three dimensions silica exhibits the very same frequency dependence at low frequencies, suggesting that this universal form is a generic consequence of amorphous glassiness.

Identifiants

pubmed: 32909803
doi: 10.1103/PhysRevLett.125.085501
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

085501

Auteurs

Silvia Bonfanti (S)

Center for Complexity and Biosystems, Department of Physics, University of Milan, via Celoria 16, 20133 Milano, Italy.

Roberto Guerra (R)

Center for Complexity and Biosystems, Department of Physics, University of Milan, via Celoria 16, 20133 Milano, Italy.

Chandana Mondal (C)

Department of Chemical Physics, The Weizmann Institute of Science, Rehovot 76100, Israel.

Itamar Procaccia (I)

Department of Chemical Physics, The Weizmann Institute of Science, Rehovot 76100, Israel.
Center for OPTical IMagery Analysis and Learning, Northwestern Polytechnical University, Xi'an, 710072 China.

Stefano Zapperi (S)

Center for Complexity and Biosystems, Department of Physics, University of Milan, via Celoria 16, 20133 Milano, Italy.
CNR-Consiglio Nazionale delle Ricerche, Istituto di Chimica della Materia Condensata e di Tecnologie per l'Energia, Via R. Cozzi 53, 20125 Milano, Italy.

Classifications MeSH