Ultrafast Carrier Relaxation Dynamics in Quantum Confined Non-Isotropic Silicon Nanostructures Synthesized by an Inductively Coupled Plasma Process.

Si nanostructure pump-probe quantum-confinement

Journal

Materials (Basel, Switzerland)
ISSN: 1996-1944
Titre abrégé: Materials (Basel)
Pays: Switzerland
ID NLM: 101555929

Informations de publication

Date de publication:
25 Sep 2020
Historique:
received: 17 08 2020
revised: 11 09 2020
accepted: 17 09 2020
entrez: 30 9 2020
pubmed: 1 10 2020
medline: 1 10 2020
Statut: epublish

Résumé

To exploit the optoelectronic properties of silicon nanostructures (SiNS) in real devices, it is fundamental to study the ultrafast processes involving the photogenerated charges separation, migration and lifetime after the optical excitation. Ultrafast time-resolved optical measurements provide such information. In the present paper, we report on the relaxation dynamics of photogenerated charge-carriers in ultrafine SiNS synthesized by means of inductively-coupled-plasma process. The carriers' transient regime was characterized in high fluence regime by using a tunable pump photon energy and a broadband probe pulse with a photon energy ranging from 1.2 eV to 2.8 eV while varying the energy of the pump photons and their polarization. The SiNS consist of Si nanospheres and nanowires (NW) with a crystalline core embedded in a SiO

Identifiants

pubmed: 32992700
pii: ma13194267
doi: 10.3390/ma13194267
pmc: PMC7579142
pii:
doi:

Types de publication

Journal Article

Langues

eng

Subventions

Organisme : Ministero degli Affari Esteri e della Cooperazione Internazionale
ID : MAE0057564

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Auteurs

Stefano Ponzoni (S)

I-Lamp and Dipartimento di Matematica e Fisica, Università Cattolica del Sacro Cuore, via dei Musei 41, 25121 Brescia, Italy.

Sonia Freddi (S)

I-Lamp and Dipartimento di Matematica e Fisica, Università Cattolica del Sacro Cuore, via dei Musei 41, 25121 Brescia, Italy.
Dipartimento di Fisica, Università degli Studi di Roma Tor Vergata, via della Ricerca Scientifica 1, 00133 Roma, Italy.

Marta Agati (M)

Dipartimento di Fisica e Astronomia, Università degli Studi di Catania, Via S. Sofia 64, 95123 Catania, Italy.
Institut National de la Recherche Scientifique, Centre-Énergie, Matériaux et Télécommunications, 1650 Blvd. Lionel-Boulet, Varennes, QC J3X-1S2, Canada.
CNR IMM-MATIS, Via S. Sofia 64, 95123 Catania, Italy.

Vincent Le Borgne (V)

Institut National de la Recherche Scientifique, Centre-Énergie, Matériaux et Télécommunications, 1650 Blvd. Lionel-Boulet, Varennes, QC J3X-1S2, Canada.

Simona Boninelli (S)

CNR IMM-MATIS, Via S. Sofia 64, 95123 Catania, Italy.

Richard Dolbec (R)

Tekna Plasma Systems Inc., 2935 Industrial Blvd., Sherbrooke, QC J1L 2T9, Canada.

My Ali El Khakani (MA)

Institut National de la Recherche Scientifique, Centre-Énergie, Matériaux et Télécommunications, 1650 Blvd. Lionel-Boulet, Varennes, QC J3X-1S2, Canada.

Stefania Pagliara (S)

I-Lamp and Dipartimento di Matematica e Fisica, Università Cattolica del Sacro Cuore, via dei Musei 41, 25121 Brescia, Italy.

Paola Castrucci (P)

Dipartimento di Fisica, Università degli Studi di Roma Tor Vergata, via della Ricerca Scientifica 1, 00133 Roma, Italy.

Classifications MeSH