The Dihydroquinolizinone Compound RG7834 Inhibits the Polyadenylase Function of PAPD5 and PAPD7 and Accelerates the Degradation of Matured Hepatitis B Virus Surface Protein mRNA.


Journal

Antimicrobial agents and chemotherapy
ISSN: 1098-6596
Titre abrégé: Antimicrob Agents Chemother
Pays: United States
ID NLM: 0315061

Informations de publication

Date de publication:
16 12 2020
Historique:
received: 02 04 2020
accepted: 30 09 2020
pubmed: 14 10 2020
medline: 22 6 2021
entrez: 13 10 2020
Statut: epublish

Résumé

Hepatitis B virus (HBV) mRNA metabolism is dependent upon host proteins PAPD5 and PAPD7 (PAPD5/7). PAPD5/7 are cellular, noncanonical, poly(A) polymerases (PAPs) whose main function is to oligoadenylate the 3' end of noncoding RNA (ncRNA) for exosome degradation. HBV seems to exploit these two ncRNA quality-control factors for viral mRNA stabilization, rather than degradation. RG7834 is a small-molecule compound that binds PAPD5/7 and inhibits HBV gene production in both tissue culture and animal study. We reported that RG7834 was able to destabilize multiple HBV mRNA species, ranging from the 3.5-kb pregenomic/precore mRNAs to the 2.4/2.1-kb hepatitis B virus surface protein (HBs) mRNAs, except for the smallest 0.7-kb X protein (HBx) mRNA. Compound-induced HBV mRNA destabilization was initiated by a shortening of the poly(A) tail, followed by an accelerated degradation process in both the nucleus and cytoplasm. In cells expressing HBV mRNA, both PAPD5/7 were found to be physically associated with the viral RNA, and the polyadenylating activities of PAPD5/7 were susceptible to RG7834 repression in a biochemical assay. Moreover, in PAPD5/7 double-knockout cells, viral transcripts with a regular length of the poly(A) sequence could be initially synthesized but became shortened in hours, suggesting that participation of PAPD5/7 in RNA 3' end processing, either during adenosine oligomerization or afterward, is crucial for RNA stabilization.

Identifiants

pubmed: 33046485
pii: AAC.00640-20
doi: 10.1128/AAC.00640-20
pmc: PMC7927841
pii:
doi:

Substances chimiques

Membrane Proteins 0
RNA, Messenger 0
RNA, Viral 0
Ribonucleases EC 3.1.-
poly A hydrolase EC 3.1.4.-

Types de publication

Journal Article Research Support, Non-U.S. Gov't

Langues

eng

Sous-ensembles de citation

IM

Informations de copyright

Copyright © 2020 American Society for Microbiology.

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Auteurs

Liren Sun (L)

Baruch S. Blumberg Institute, Department of Translational Medicine, Doylestown, Pennsylvania, USA.

Fang Zhang (F)

Baruch S. Blumberg Institute, Department of Translational Medicine, Doylestown, Pennsylvania, USA.

Fang Guo (F)

Arbutus BioPharma, Warminster, Pennsylvania, USA.

Fei Liu (F)

Arbutus BioPharma, Warminster, Pennsylvania, USA.

Jessie Kulsuptrakul (J)

Chan Zuckerberg Biohub, San Francisco, California, USA.

Andreas Puschnik (A)

Chan Zuckerberg Biohub, San Francisco, California, USA.

Min Gao (M)

Arbutus BioPharma, Warminster, Pennsylvania, USA.

Rene Rijnbrand (R)

Arbutus BioPharma, Warminster, Pennsylvania, USA.

Michael Sofia (M)

Arbutus BioPharma, Warminster, Pennsylvania, USA.

Timothy Block (T)

Baruch S. Blumberg Institute, Department of Translational Medicine, Doylestown, Pennsylvania, USA tim.block@bblumberg.org tianlun.zhou@bblumberg.org.

Tianlun Zhou (T)

Baruch S. Blumberg Institute, Department of Translational Medicine, Doylestown, Pennsylvania, USA tim.block@bblumberg.org tianlun.zhou@bblumberg.org.

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Classifications MeSH