Analysis of protein-DNA interactions in chromatin by UV induced cross-linking and mass spectrometry.


Journal

Nature communications
ISSN: 2041-1723
Titre abrégé: Nat Commun
Pays: England
ID NLM: 101528555

Informations de publication

Date de publication:
16 10 2020
Historique:
received: 06 09 2019
accepted: 24 09 2020
entrez: 17 10 2020
pubmed: 18 10 2020
medline: 18 11 2020
Statut: epublish

Résumé

Protein-DNA interactions are key to the functionality and stability of the genome. Identification and mapping of protein-DNA interaction interfaces and sites is crucial for understanding DNA-dependent processes. Here, we present a workflow that allows mass spectrometric (MS) identification of proteins in direct contact with DNA in reconstituted and native chromatin after cross-linking by ultraviolet (UV) light. Our approach enables the determination of contact interfaces at amino-acid level. With the example of chromatin-associated protein SCML2 we show that our technique allows differentiation of nucleosome-binding interfaces in distinct states. By UV cross-linking of isolated nuclei we determined the cross-linking sites of several factors including chromatin-modifying enzymes, demonstrating that our workflow is not restricted to reconstituted materials. As our approach can distinguish between protein-RNA and DNA interactions in one single experiment, we project that it will be possible to obtain insights into chromatin and its regulation in the future.

Identifiants

pubmed: 33067435
doi: 10.1038/s41467-020-19047-7
pii: 10.1038/s41467-020-19047-7
pmc: PMC7567871
doi:

Substances chimiques

Chromatin 0
Nucleosomes 0
Polycomb-Group Proteins 0
Proteins 0
SCML2 protein, human 0
DNA 9007-49-2

Types de publication

Journal Article Research Support, Non-U.S. Gov't

Langues

eng

Sous-ensembles de citation

IM

Pagination

5250

Subventions

Organisme : Wellcome Trust
Pays : United Kingdom
Organisme : Medical Research Council
Pays : United Kingdom
Organisme : Wellcome Trust
ID : 109854/Z/15/Z
Pays : United Kingdom

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Auteurs

Alexandra Stützer (A)

Bioanalytical Mass Spectrometry Group, Max Planck Institute for Biophysical Chemistry, 37077, Göttingen, Germany.

Luisa M Welp (LM)

Bioanalytical Mass Spectrometry Group, Max Planck Institute for Biophysical Chemistry, 37077, Göttingen, Germany.

Monika Raabe (M)

Bioanalytical Mass Spectrometry Group, Max Planck Institute for Biophysical Chemistry, 37077, Göttingen, Germany.

Timo Sachsenberg (T)

Institute for Bioinformatics and Medical Informatics, University of Tübingen, 72076, Tübingen, Germany.
Applied Bioinformatics, Department for Computer Science, University of Tübingen, 72076, Tübingen, Germany.

Christin Kappert (C)

Bioanalytical Mass Spectrometry Group, Max Planck Institute for Biophysical Chemistry, 37077, Göttingen, Germany.
Somatosensory Signaling and Systems Biology Group, Max Planck Institute of Experimental Medicine, 37075, Göttingen, Germany.

Alexander Wulf (A)

Bioanalytical Mass Spectrometry Group, Max Planck Institute for Biophysical Chemistry, 37077, Göttingen, Germany.

Andy M Lau (AM)

Department of Chemistry, King's College London, London, SE1 1DB, UK.

Stefan-Sebastian David (SS)

Laboratory of Chromatin Biochemistry, Max Planck Institute for Biophysical Chemistry, 37077, Göttingen, Germany.
King Abdullah University of Science and Technology (KAUST), Biological and Environmental Science and Engineering Division, Laboratory of Chromatin Biochemistry, 23955, Thuwal, Saudi Arabia.

Aleksandar Chernev (A)

Bioanalytical Mass Spectrometry Group, Max Planck Institute for Biophysical Chemistry, 37077, Göttingen, Germany.

Katharina Kramer (K)

CSL Behring GmbH, 35041, Marburg, Germany.

Argyris Politis (A)

Department of Chemistry, King's College London, London, SE1 1DB, UK.

Oliver Kohlbacher (O)

Institute for Bioinformatics and Medical Informatics, University of Tübingen, 72076, Tübingen, Germany.
Applied Bioinformatics, Department for Computer Science, University of Tübingen, 72076, Tübingen, Germany.
Institute for Translational Bioinformatics, University Hospital Tübingen, 72076, Tübingen, Germany.
Biomolecular Interactions, Max Planck Institute for Developmental Biology, 72076, Tübingen, Germany.

Wolfgang Fischle (W)

Laboratory of Chromatin Biochemistry, Max Planck Institute for Biophysical Chemistry, 37077, Göttingen, Germany.
King Abdullah University of Science and Technology (KAUST), Biological and Environmental Science and Engineering Division, Laboratory of Chromatin Biochemistry, 23955, Thuwal, Saudi Arabia.

Henning Urlaub (H)

Bioanalytical Mass Spectrometry Group, Max Planck Institute for Biophysical Chemistry, 37077, Göttingen, Germany. henning.urlaub@mpibpc.mpg.de.
Bioanalytics Group, Institute for Clinical Chemistry, University Medical Center Göttingen, 37075, Göttingen, Germany. henning.urlaub@mpibpc.mpg.de.

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Classifications MeSH