Development of Ligand-Drug Conjugates Targeting Melanoma through the Overexpressed Melanocortin 1 Receptor.


Journal

ACS pharmacology & translational science
ISSN: 2575-9108
Titre abrégé: ACS Pharmacol Transl Sci
Pays: United States
ID NLM: 101721411

Informations de publication

Date de publication:
09 Oct 2020
Historique:
received: 23 06 2020
entrez: 19 10 2020
pubmed: 20 10 2020
medline: 20 10 2020
Statut: epublish

Résumé

Melanoma is a lethal form of skin cancer. Despite recent breakthroughs of BRAF-V600E and PD-1 inhibitors showing remarkable clinical responses, melanoma can eventually survive these targeted therapies and become resistant. To solve the drug resistance issue, we designed and synthesized ligand-drug conjugates that couple cytotoxic drugs, which have a low cancer resistance issue, with the melanocortin 1 receptor (MC1R) agonist melanotan-II (MT-II), which provides specificity to MC1R-overexpressing melanoma. The drug-MT-II conjugates maintain strong binding interactions to MC1R and induce selective drug delivery to A375 melanoma cells through its MT-II moiety

Identifiants

pubmed: 33073191
doi: 10.1021/acsptsci.0c00072
pmc: PMC7551717
doi:

Types de publication

Journal Article

Langues

eng

Pagination

921-930

Subventions

Organisme : NIDDK NIH HHS
ID : R01 DK017420
Pays : United States
Organisme : NIGMS NIH HHS
ID : R01 GM108040
Pays : United States

Déclaration de conflit d'intérêts

The authors declare no competing financial interest.

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Auteurs

Yang Zhou (Y)

Department of Chemistry and Biochemistry, The University of Arizona, Tucson, Arizona 85721, United States.

Saghar Mowlazadeh Haghighi (S)

Department of Chemistry and Biochemistry, The University of Arizona, Tucson, Arizona 85721, United States.

Zekun Liu (Z)

Department of Chemistry and Biochemistry, The University of Arizona, Tucson, Arizona 85721, United States.

Lingzhi Wang (L)

Department of Chemistry and Biochemistry, The University of Arizona, Tucson, Arizona 85721, United States.

Victor J Hruby (VJ)

Department of Chemistry and Biochemistry, The University of Arizona, Tucson, Arizona 85721, United States.

Minying Cai (M)

Department of Chemistry and Biochemistry, The University of Arizona, Tucson, Arizona 85721, United States.

Classifications MeSH