Total Synthesis of the Diterpene Waihoensene.

Pauson-Khand reaction natural products radicals terpenes total synthesis

Journal

Angewandte Chemie (International ed. in English)
ISSN: 1521-3773
Titre abrégé: Angew Chem Int Ed Engl
Pays: Germany
ID NLM: 0370543

Informations de publication

Date de publication:
08 02 2021
Historique:
received: 18 08 2020
pubmed: 27 10 2020
medline: 27 10 2020
entrez: 26 10 2020
Statut: ppublish

Résumé

A racemic and scalable enantioselective total synthesis of (+)-waihoensene was accomplished. (+)-Waihoensene belongs to the diterpene natural product family, and it features an angular triquinane substructure motif. Its tetracyclic [6.5.5.5]backbone is all-cis-fused, containing six contiguous stereocenters, four of which are quaternary. These structural features were efficiently installed by means of a diastereoselective radical cyclization, followed by an intramolecular Pauson-Khand reaction, a diastereoselective α-alkylation, and a diastereoselective 1,4-addition reaction. Enantioselectivity was introduced at an early stage, by an asymmetric palladium catalyzed decarboxylative allylation reaction on gram scale.

Identifiants

pubmed: 33103334
doi: 10.1002/anie.202011298
pmc: PMC7898921
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

2939-2942

Informations de copyright

© 2020 The Authors. Angewandte Chemie International Edition published by Wiley-VCH GmbH.

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Auteurs

Lisa-Catherine Rosenbaum (LC)

Department of Chemistry, University of Konstanz, Universitätsstrasse 10, 78464, Konstanz, Germany.

Maximilian Häfner (M)

Department of Chemistry, University of Konstanz, Universitätsstrasse 10, 78464, Konstanz, Germany.

Tanja Gaich (T)

Department of Chemistry, University of Konstanz, Universitätsstrasse 10, 78464, Konstanz, Germany.

Classifications MeSH