PLGA Membranes Functionalized with Gelatin through Biomimetic Mussel-Inspired Strategy.

DOPA PLGA biomimetic functionalization electrospinning surface modification

Journal

Nanomaterials (Basel, Switzerland)
ISSN: 2079-4991
Titre abrégé: Nanomaterials (Basel)
Pays: Switzerland
ID NLM: 101610216

Informations de publication

Date de publication:
02 Nov 2020
Historique:
received: 30 07 2020
revised: 16 09 2020
accepted: 29 10 2020
entrez: 5 11 2020
pubmed: 6 11 2020
medline: 6 11 2020
Statut: epublish

Résumé

Electrospun membranes have been widely used as scaffolds for soft tissue engineering due to their extracellular matrix-like structure. A mussel-inspired coating approach based on 3,4-dihydroxy-DL-phenylalanine (DOPA) polymerization was proposed to graft gelatin (G) onto poly(lactic-co-glycolic) acid (PLGA) electrospun membranes. PolyDOPA coating allowed grafting of gelatin to PLGA fibers without affecting their bulk characteristics, such as molecular weight and thermal properties. PLGA electrospun membranes were dipped in a DOPA solution (2 mg/mL, Tris/HCl 10 mM, pH 8.5) for 7 h and then incubated in G solution (2 mg/mL, Tris/HCl 10 mM, pH 8.5) for 16 h. PLGA fibers had an average diameter of 1.37 ± 0.23 µm. Quartz crystal microbalance with dissipation technique (QCM-D) analysis was performed to monitor DOPA polymerization over time: after 7 h the amount of deposited polyDOPA was 71 ng/cm

Identifiants

pubmed: 33147761
pii: nano10112184
doi: 10.3390/nano10112184
pmc: PMC7692787
pii:
doi:

Types de publication

Journal Article

Langues

eng

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Auteurs

Irene Carmagnola (I)

Department of Mechanical and Aerospace Engineering, Politecnico di Torino, 10129 Torino, Italy.
POLITO BIOMedLAB, Politecnico di Torino, 10129 Turin, Italy.

Valeria Chiono (V)

Department of Mechanical and Aerospace Engineering, Politecnico di Torino, 10129 Torino, Italy.
POLITO BIOMedLAB, Politecnico di Torino, 10129 Turin, Italy.
Department for Materials and Devices of the National Research Council, Institute for the Chemical and Physical Processes (CNR-IPCF UOS), 56124 Pisa, Italy.

Gerardina Ruocco (G)

Department of Mechanical and Aerospace Engineering, Politecnico di Torino, 10129 Torino, Italy.
POLITO BIOMedLAB, Politecnico di Torino, 10129 Turin, Italy.

Annachiara Scalzone (A)

School of Engineering, Newcastle University, Claremont road, Newcastle upon Tyne NE1 7RU, UK.

Piergiorgio Gentile (P)

School of Engineering, Newcastle University, Claremont road, Newcastle upon Tyne NE1 7RU, UK.

Paola Taddei (P)

Department of Biomedical and Neuromotor Sciences, University of Bologna, 40126 Bologna, Italy.

Gianluca Ciardelli (G)

Department of Mechanical and Aerospace Engineering, Politecnico di Torino, 10129 Torino, Italy.
POLITO BIOMedLAB, Politecnico di Torino, 10129 Turin, Italy.
Department for Materials and Devices of the National Research Council, Institute for the Chemical and Physical Processes (CNR-IPCF UOS), 56124 Pisa, Italy.

Classifications MeSH