Elucidation of Gut Microbiota-Associated Lipids Using LC-MS/MS and 16S rRNA Sequence Analyses.

Lipidomics Microbiome Omics

Journal

iScience
ISSN: 2589-0042
Titre abrégé: iScience
Pays: United States
ID NLM: 101724038

Informations de publication

Date de publication:
18 Dec 2020
Historique:
received: 03 07 2020
revised: 25 10 2020
accepted: 18 11 2020
entrez: 14 12 2020
pubmed: 15 12 2020
medline: 15 12 2020
Statut: epublish

Résumé

Host-microbiota interactions create a unique metabolic milieu that modulates intestinal environments. Integration of 16S ribosomal RNA (rRNA) sequences and mass spectrometry (MS)-based lipidomics has a great potential to reveal the relationship between bacterial composition and the complex metabolic network in the gut. In this study, we conducted untargeted lipidomics followed by a feature-based molecular MS/MS spectral networking to characterize gut bacteria-dependent lipid subclasses in mice. An estimated 24.8% of lipid molecules in feces were microbiota-dependent, as judged by > 10-fold decrease in antibiotic-treated mice. Among these, there was a series of unique and microbiota-related lipid structures, including acyl alpha-hydroxyl fatty acid (AAHFA) that was newly identified in this study

Identifiants

pubmed: 33313490
doi: 10.1016/j.isci.2020.101841
pii: S2589-0042(20)31038-5
pmc: PMC7721639
doi:

Types de publication

Journal Article

Langues

eng

Pagination

101841

Informations de copyright

© 2020 The Author(s).

Déclaration de conflit d'intérêts

The authors declare no competing interests.

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Auteurs

Shu Yasuda (S)

RIKEN Center for Integrative Medical Sciences, Yokohama 230-0045, Japan.
Department of Health Chemistry, Graduate School of Pharmaceutical Sciences, University of Tokyo, 7-3-1, Hongo, Bunkyo-ku, Tokyo 113-0033, Japan.

Nobuyuki Okahashi (N)

RIKEN Center for Integrative Medical Sciences, Yokohama 230-0045, Japan.
Graduate School of Information Science and Technology, Osaka University, 1-5 Yamadaoka, Suita, Osaka 565-0871, Japan.

Hiroshi Tsugawa (H)

RIKEN Center for Integrative Medical Sciences, Yokohama 230-0045, Japan.
RIKEN Center for Sustainable Resource Science, Yokohama 230-0045, Japan.

Yusuke Ogata (Y)

RIKEN Center for Integrative Medical Sciences, Yokohama 230-0045, Japan.

Kazutaka Ikeda (K)

RIKEN Center for Integrative Medical Sciences, Yokohama 230-0045, Japan.
Clinical Omics Unit, Kazusa DNA Research Institute, Kisarazu, Chiba, Japan.

Wataru Suda (W)

RIKEN Center for Integrative Medical Sciences, Yokohama 230-0045, Japan.

Hiroyuki Arai (H)

Department of Health Chemistry, Graduate School of Pharmaceutical Sciences, University of Tokyo, 7-3-1, Hongo, Bunkyo-ku, Tokyo 113-0033, Japan.

Masahira Hattori (M)

RIKEN Center for Integrative Medical Sciences, Yokohama 230-0045, Japan.
Faculty of Science and Engineering, Waseda University, 3-4-1 Okubo, Shinjuku-ku, Tokyo 169-8555, Japan.

Makoto Arita (M)

RIKEN Center for Integrative Medical Sciences, Yokohama 230-0045, Japan.
Division of Physiological Chemistry and Metabolism, Graduate School of Pharmaceutical Sciences, Keio University, Minato-ku, Tokyo 105-8512, Japan.
Graduate School of Medical Life Science, Yokohama City University, Tsurumi, Yokohama 230-0045, Japan.

Classifications MeSH