Spent Li-Ion Battery Graphite Turned Into Valuable and Active Catalyst for Electrochemical Oxygen Reduction.
circular economy
graphene oxide
nitrogen-doped graphene
oxygen reduction reaction
recycling of Li-ion battery
Journal
ChemSusChem
ISSN: 1864-564X
Titre abrégé: ChemSusChem
Pays: Germany
ID NLM: 101319536
Informations de publication
Date de publication:
18 Feb 2021
18 Feb 2021
Historique:
received:
27
11
2020
pubmed:
15
12
2020
medline:
15
12
2020
entrez:
14
12
2020
Statut:
ppublish
Résumé
Employing Li-ion batteries (LIBs) in portable electronics has become a necessity in the modern world but, due to the short application time for any given battery (1-3 years), the quantity of spent LIBs (SLIBs) waste is becoming substantial. Herein, a novel strategy for recycling SLIB graphite and reforming it as a valuable catalyst material for electrochemical oxygen reduction reaction was proposed. SLIB graphite has been used as a precursor material for graphite oxide, which was thereafter doped with nitrogen to prepare nitrogen-doped graphene (NG-Bat). The prepared NG-Bat was characterized by various physical characterization methods and the electrochemical properties of the resulting catalyst material were investigated in alkaline media. It was found that NG-Bat prepared from SLIB had superior physical and electrochemical properties in comparison to commercial nitrogen-doped graphene. The findings clearly demonstrate the importance of the recycling of SLIB graphite and its great potential to be re-applied for various applications.
Identifiants
pubmed: 33314598
doi: 10.1002/cssc.202002742
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
1103-1111Subventions
Organisme : Estonian Research Council
ID : PSG312
Organisme : Estonian Research Council
ID : IUT19-28
Organisme : Estonian Research Council
ID : TK-141
Organisme : ERA.Net RUS
ID : HeDoCat
Organisme : European Regional Development Fund
ID : 2014-2020.4.01.16-0041
Organisme : European Regional Development Fund
ID : 2014-2020.4.01.15-0005
Organisme : University of California at Berkeley
Informations de copyright
© 2020 Wiley-VCH GmbH.
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