Observing the Structural Evolution in the Photodissociation of Diiodomethane with Femtosecond Solution X-Ray Scattering.


Journal

Physical review letters
ISSN: 1079-7114
Titre abrégé: Phys Rev Lett
Pays: United States
ID NLM: 0401141

Informations de publication

Date de publication:
27 Nov 2020
Historique:
received: 19 08 2020
revised: 25 09 2020
accepted: 19 10 2020
entrez: 14 12 2020
pubmed: 15 12 2020
medline: 15 12 2020
Statut: ppublish

Résumé

Resolving the structural dynamics of the initial steps of chemical reactions is challenging. We report the femtosecond time-resolved wide-angle x-ray scattering of the photodissociation of diiodomethane in cyclohexane. The data reveal with structural detail how the molecule dissociates into radicals, how the radicals collide with the solvent, and how they form the photoisomer. We extract how translational and rotational kinetic energy is dispersed into the solvent. We also find that 85% of the primary radical pairs are confined to their original solvent cage and discuss how this influences the downstream recombination reactions.

Identifiants

pubmed: 33315438
doi: 10.1103/PhysRevLett.125.226001
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

226001

Auteurs

Matthijs R Panman (MR)

Department of Chemistry and Molecular Biology, University of Gothenburg, Box 462, 40530 Gothenburg, Sweden.

Elisa Biasin (E)

Centre for Molecular Movies, Department of Physics, Technical University of Denmark, DK-2800 Lyngby, Denmark.

Oskar Berntsson (O)

Department of Chemistry and Molecular Biology, University of Gothenburg, Box 462, 40530 Gothenburg, Sweden.

Markus Hermann (M)

Georg-August-Universität Göttingen, Institute for Microbiology and Genetics, Justus-von-Liebig-Weg 11, 37077 Göttingen, Germany.

Stephan Niebling (S)

Department of Chemistry and Molecular Biology, University of Gothenburg, Box 462, 40530 Gothenburg, Sweden.

Ashley J Hughes (AJ)

Department of Chemistry and Molecular Biology, University of Gothenburg, Box 462, 40530 Gothenburg, Sweden.

Joachim Kübel (J)

Department of Chemistry and Molecular Biology, University of Gothenburg, Box 462, 40530 Gothenburg, Sweden.

Kalina Atkovska (K)

Georg-August-Universität Göttingen, Institute for Microbiology and Genetics, Justus-von-Liebig-Weg 11, 37077 Göttingen, Germany.

Emil Gustavsson (E)

Department of Chemistry and Molecular Biology, University of Gothenburg, Box 462, 40530 Gothenburg, Sweden.

Amke Nimmrich (A)

Department of Chemistry and Molecular Biology, University of Gothenburg, Box 462, 40530 Gothenburg, Sweden.

Asmus O Dohn (AO)

Centre for Molecular Movies, Department of Physics, Technical University of Denmark, DK-2800 Lyngby, Denmark.

Mads Laursen (M)

Centre for Molecular Movies, Department of Physics, Technical University of Denmark, DK-2800 Lyngby, Denmark.

Diana B Zederkof (DB)

Centre for Molecular Movies, Department of Physics, Technical University of Denmark, DK-2800 Lyngby, Denmark.

Alireza Honarfar (A)

Department of Chemical Physics, Lund University, Box 124, S-2210, Lund, Sweden.

Kensuke Tono (K)

Japan Synchrotron Radiation Research Institute, 1-1-1 Kouto, Sayo-cho, Sayo-gun, Hyogo 679-5198, Japan.

Tetsuo Katayama (T)

Japan Synchrotron Radiation Research Institute, 1-1-1 Kouto, Sayo-cho, Sayo-gun, Hyogo 679-5198, Japan.

Shigeki Owada (S)

RIKEN SPring-8 Center, 1-1-1 Kouto, Sayo-cho, Sayo-gun, Hyogo 679-5148, Japan.

Tim B van Driel (TB)

LCLS, SLAC National Laboratory, Menlo Park, California 94025, USA.

Kasper Kjaer (K)

LCLS, SLAC National Laboratory, Menlo Park, California 94025, USA.

Martin M Nielsen (MM)

Centre for Molecular Movies, Department of Physics, Technical University of Denmark, DK-2800 Lyngby, Denmark.

Jan Davidsson (J)

Department of Chemistry, Ångström Laboratory, Uppsala University, Box 523, SE75120 Uppsala, Sweden.

Jens Uhlig (J)

Department of Chemical Physics, Lund University, Box 124, S-2210, Lund, Sweden.

Kristoffer Haldrup (K)

Centre for Molecular Movies, Department of Physics, Technical University of Denmark, DK-2800 Lyngby, Denmark.

Jochen S Hub (JS)

Georg-August-Universität Göttingen, Institute for Microbiology and Genetics, Justus-von-Liebig-Weg 11, 37077 Göttingen, Germany.

Sebastian Westenhoff (S)

Department of Chemistry and Molecular Biology, University of Gothenburg, Box 462, 40530 Gothenburg, Sweden.

Classifications MeSH