Self-Assembly of Metallo-Supramolecules with Dissymmetrical Ligands and Characterization by Scanning Tunneling Microscopy.

Journal

Journal of the American Chemical Society
ISSN: 1520-5126
Titre abrégé: J Am Chem Soc
Pays: United States
ID NLM: 7503056

Informations de publication

Date de publication:
20 01 2021
Historique:
pubmed: 5 1 2021
medline: 5 1 2021
entrez: 4 1 2021
Statut: ppublish

Résumé

Asymmetrical and dissymmetrical structures are widespread and play a critical role in nature and life systems. In the field of metallo-supramolecular assemblies, it is still in its infancy for constructing artificial architectures using dissymmetrical building blocks. Herein, we report the self-assembly of supramolecular systems based on two dissymmetrical double-layered ligands. With the aid of ultra-high-vacuum, low-temperature scanning tunneling microscopy (UHV-LT-STM), we were able to investigate four isomeric structures corresponding to four types of binding modes of ligand

Identifiants

DOI: 10.1021/jacs.0c12508 PMID: 33395279
pubmed: 33395279
doi: 10.1021/jacs.0c12508
doi:

Types de publication

Journal Article Research Support, Non-U.S. Gov't

Langues

eng

Sous-ensembles de citation

IM

Pagination

1224-1234

Auteurs

Junjuan Shi (J)

State Key Laboratory of Supramolecular Structure and Materials, College of Chemistry, Jilin University, Changchun, Jilin 130012, China.
College of Chemistry and Environmental Engineering, Shenzhen University, Shenzhen, Guangdong 518055, China.

Yiming Li (Y)

College of Chemistry and Environmental Engineering, Shenzhen University, Shenzhen, Guangdong 518055, China.
Department of Chemistry, University of South Florida, Tampa, Florida 33620, United States.

Xin Jiang (X)

State Key Laboratory of Supramolecular Structure and Materials, College of Chemistry, Jilin University, Changchun, Jilin 130012, China.

Hao Yu (H)

State Key Laboratory of Supramolecular Structure and Materials, College of Chemistry, Jilin University, Changchun, Jilin 130012, China.

Jiaqi Li (J)

State Key Laboratory of Supramolecular Structure and Materials, College of Chemistry, Jilin University, Changchun, Jilin 130012, China.

Houyu Zhang (H)

State Key Laboratory of Supramolecular Structure and Materials, College of Chemistry, Jilin University, Changchun, Jilin 130012, China.
ORCID: 0000-0003-0360-6035

Daniel J Trainer (DJ)

Nanoscience and Technology Division, Argonne National Laboratory, Lemont, Illinois 60439, United States.

Saw Wai Hla (SW)

Nanoscience and Technology Division, Argonne National Laboratory, Lemont, Illinois 60439, United States.

Heng Wang (H)

College of Chemistry and Environmental Engineering, Shenzhen University, Shenzhen, Guangdong 518055, China.

Ming Wang (M)

State Key Laboratory of Supramolecular Structure and Materials, College of Chemistry, Jilin University, Changchun, Jilin 130012, China.
ORCID: 0000-0002-5332-0804

Xiaopeng Li (X)

College of Chemistry and Environmental Engineering, Shenzhen University, Shenzhen, Guangdong 518055, China.
Shenzhen University General Hospital, Clinical Medical Academy, Shenzhen University, Shenzhen, Guangdong 518055, China.
ORCID: 0000-0001-9655-9551

Classifications MeSH