Halogen-Imparted Reactivity in Lithium Carbenoid Mediated Homologations of Imine Surrogates: Direct Assembly of bis-Trifluoromethyl-β-Diketiminates and the Dual Role of LiCH

carbenoids chemoselectivity homologation imines metalation

Journal

Angewandte Chemie (International ed. in English)
ISSN: 1521-3773
Titre abrégé: Angew Chem Int Ed Engl
Pays: Germany
ID NLM: 0370543

Informations de publication

Date de publication:
16 11 2020
Historique:
received: 03 06 2020
revised: 17 07 2020
entrez: 15 1 2021
pubmed: 16 1 2021
medline: 16 1 2021
Statut: ppublish

Résumé

The selective formal insertion (homologation) of a carbon unit bridging the two trifluoroacetamidoyl chlorides (TFAICs) units is reported. The tactic is levered on a highly chemoselective homologation-metalation-acyl nucleophilic substitution sequence which precisely enables to assemble novel trifluoromethylated β-diketiminates within a single synthetic operation. Unlike previous homologations conducted with LiCH

Identifiants

pubmed: 33448561
doi: 10.1002/anie.202007954
doi:

Types de publication

Journal Article Research Support, Non-U.S. Gov't

Langues

eng

Sous-ensembles de citation

IM

Pagination

20852-20857

Informations de copyright

© 2020 Wiley‐VCH GmbH.

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Auteurs

Laura Ielo (L)

University of Vienna, Department of Pharmaceutical Chemistry, Althanstrasse 14, 1090, Vienna, Austria.

Laura Castoldi (L)

University of Vienna, Department of Pharmaceutical Chemistry, Althanstrasse 14, 1090, Vienna, Austria.

Saad Touqeer (S)

University of Vienna, Department of Pharmaceutical Chemistry, Althanstrasse 14, 1090, Vienna, Austria.

Jessica Lombino (J)

Fondazione Ri.MED, Via Bandiera 11, 90133, Palermo, Italy.
University of Palermo, Department STEBICEF, Via Archirafi 32, 90123, Palermo, Italy.

Alexander Roller (A)

University of Vienna, X-Ray Structure Analysis Center, Waehringerstrasse 42, 1090, Vienna, Austria.

Cristina Prandi (C)

University of Turin, Department of Chemistry, Via P. Giuria 7, 10125, Turin, Italy.

Wolfgang Holzer (W)

University of Vienna, Department of Pharmaceutical Chemistry, Althanstrasse 14, 1090, Vienna, Austria.

Vittorio Pace (V)

University of Vienna, Department of Pharmaceutical Chemistry, Althanstrasse 14, 1090, Vienna, Austria.
University of Turin, Department of Chemistry, Via P. Giuria 7, 10125, Turin, Italy.

Classifications MeSH