How volatile components catalyze vapor nucleation.


Journal

Science advances
ISSN: 2375-2548
Titre abrégé: Sci Adv
Pays: United States
ID NLM: 101653440

Informations de publication

Date de publication:
Jan 2021
Historique:
received: 24 07 2020
accepted: 16 11 2020
entrez: 1 2 2021
pubmed: 2 2 2021
medline: 2 2 2021
Statut: epublish

Résumé

Gas phase nucleation is a ubiquitous phenomenon in planetary atmospheres and technical processes, yet our understanding of it is far from complete. In particular, the enhancement of nucleation by the addition of a more volatile, weakly interacting gaseous species to a nucleating vapor has escaped molecular-level experimental investigation. Here, we use a specially designed experiment to directly measure the chemical composition and the concentration of nucleating clusters in various binary CO

Identifiants

pubmed: 33523884
pii: 7/3/eabd9954
doi: 10.1126/sciadv.abd9954
pmc: PMC7806218
pii:
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Informations de copyright

Copyright © 2021 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution NonCommercial License 4.0 (CC BY-NC).

Références

Phys Chem Chem Phys. 2005 Jul 21;7(14):2764-70
pubmed: 16189591
Science. 2004 Jun 4;304(5676):1487-90
pubmed: 15178797
Science. 2016 Dec 2;354(6316):1119-1124
pubmed: 27789796
Proc Natl Acad Sci U S A. 2014 Oct 21;111(42):15019-24
pubmed: 25288761
Chem Commun (Camb). 2019 May 25;55(42):5946-5949
pubmed: 31049542
J Phys Chem A. 2007 Oct 11;111(40):10075-83
pubmed: 17715907
Science. 2018 Jul 20;361(6399):278-281
pubmed: 30026225
J Phys Chem A. 2019 Mar 28;123(12):2426-2437
pubmed: 30835464
J Chem Phys. 2019 Dec 28;151(24):244202
pubmed: 31893907
Phys Chem Chem Phys. 2019 Apr 17;21(16):8295-8313
pubmed: 30946401
Phys Chem Chem Phys. 2013 Jan 21;15(3):940-9
pubmed: 23201898
J Chem Phys. 2018 Dec 28;149(24):244303
pubmed: 30599746
Phys Chem Chem Phys. 2020 Jul 22;22(28):15986-15998
pubmed: 32632423
J Phys Chem A. 2017 May 25;121(20):3991-4001
pubmed: 28481529
J Chem Phys. 2019 Sep 7;151(9):094305
pubmed: 31492059
J Phys Chem A. 2016 Mar 24;120(11):1886-96
pubmed: 26918813
J Chem Phys. 2016 Dec 7;145(21):211907
pubmed: 28799355
Proc Natl Acad Sci U S A. 2018 Sep 11;115(37):9122-9127
pubmed: 30154167
Mass Spectrom Rev. 2018 Sep;37(5):630-651
pubmed: 29178389
Nat Chem. 2013 Sep;5(9):745-9
pubmed: 23965675
J Phys Chem A. 2019 Jan 17;123(2):611-624
pubmed: 30550283
Science. 2014 May 16;344(6185):717-21
pubmed: 24833386
Proc Natl Acad Sci U S A. 2012 Nov 13;109(46):18713-8
pubmed: 23091030
J Phys Chem A. 2016 Mar 10;120(9):1452-8
pubmed: 26544764
Phys Chem Chem Phys. 2015 Oct 21;17(39):25761-71
pubmed: 25792194
Phys Rev Lett. 2016 Mar 18;116(11):113401
pubmed: 27035301
Chemphyschem. 2007 Feb 19;8(3):343-56
pubmed: 17290359

Auteurs

Chenxi Li (C)

School of Environmental Science and Engineering, Shanghai Jiao Tong University, Shanghai 200240, China.
Department of Chemistry and Applied Biosciences, Laboratory of Physical Chemistry, ETH Zürich, Vladimir-Prelog-Weg 2, CH-8093 Zürich, Switzerland.

Jan Krohn (J)

Department of Chemistry and Applied Biosciences, Laboratory of Physical Chemistry, ETH Zürich, Vladimir-Prelog-Weg 2, CH-8093 Zürich, Switzerland.

Martina Lippe (M)

Department of Chemistry and Applied Biosciences, Laboratory of Physical Chemistry, ETH Zürich, Vladimir-Prelog-Weg 2, CH-8093 Zürich, Switzerland.

Ruth Signorell (R)

Department of Chemistry and Applied Biosciences, Laboratory of Physical Chemistry, ETH Zürich, Vladimir-Prelog-Weg 2, CH-8093 Zürich, Switzerland. rsignorell@ethz.ch.

Classifications MeSH