Suzuki Coupling of Protected Aryl Diazonium Ions: Expanding the Knowledge of Triazabutadiene Compatible Reactions.


Journal

Organic letters
ISSN: 1523-7052
Titre abrégé: Org Lett
Pays: United States
ID NLM: 100890393

Informations de publication

Date de publication:
05 03 2021
Historique:
pubmed: 12 2 2021
medline: 5 10 2021
entrez: 11 2 2021
Statut: ppublish

Résumé

Aryl diazonium ions are important in synthesis and chemical biology, and the acid-labile triazabutadiene can protect this handle for future use. We report a Suzuki coupling strategy that is compatible with the triazabutadiene scaffold, expanding the scope of synthetically available triazabutadienes. Shown herein, the triazabutadiene scaffold remains intact and reactive after coupling, as demonstrated by releasing the aryl diazonium ion to label a tyrosine-rich model protein.

Identifiants

pubmed: 33570414
doi: 10.1021/acs.orglett.1c00257
pmc: PMC7955896
mid: NIHMS1675740
doi:

Substances chimiques

Diazonium Compounds 0
Ions 0
Proteins 0

Types de publication

Journal Article Research Support, N.I.H., Extramural Research Support, Non-U.S. Gov't Research Support, U.S. Gov't, Non-P.H.S.

Langues

eng

Sous-ensembles de citation

IM

Pagination

1851-1855

Subventions

Organisme : NIGMS NIH HHS
ID : R35 GM128624
Pays : United States
Organisme : NIGMS NIH HHS
ID : T32 GM008804
Pays : United States

Références

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Auteurs

Abigail J Shepard (AJ)

Department of Pharmacology and Toxicology, University of Arizona, Tucson, Arizona 85721, United States.
Department of Chemistry and Biochemistry, University of Arizona, Tucson, Arizona 85721, United States.

Julia A Townsend (JA)

Department of Chemistry and Biochemistry, University of Arizona, Tucson, Arizona 85721, United States.

Christopher Foley (C)

Department of Pharmacology and Toxicology, University of Arizona, Tucson, Arizona 85721, United States.
Department of Chemistry and Biochemistry, University of Arizona, Tucson, Arizona 85721, United States.

Christopher Hulme (C)

Department of Pharmacology and Toxicology, University of Arizona, Tucson, Arizona 85721, United States.

Michael T Marty (MT)

Department of Chemistry and Biochemistry, University of Arizona, Tucson, Arizona 85721, United States.

John C Jewett (JC)

Department of Chemistry and Biochemistry, University of Arizona, Tucson, Arizona 85721, United States.

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Classifications MeSH