Development of novel multifunctional adsorbent by effectively hosting both zwitterionic surfactant and hydrated ferric oxides in montmorillonite.

Interlayer space Montmorillonite Multifunctional adsorbent Tetrachloroferrate Zwitterionic surfactant

Journal

The Science of the total environment
ISSN: 1879-1026
Titre abrégé: Sci Total Environ
Pays: Netherlands
ID NLM: 0330500

Informations de publication

Date de publication:
20 Jun 2021
Historique:
received: 20 10 2020
revised: 21 12 2020
accepted: 01 01 2021
pubmed: 22 2 2021
medline: 22 2 2021
entrez: 21 2 2021
Statut: ppublish

Résumé

Intercalating various functional species into the interlayer space is an effective strategy to multi-functionalize 2D materials (e.g., montmorillonite, Mnt), but general limitations have emerged therefrom: (1) various intercalated species compete for the limited interlayer space, and (2) the neighboring intercalated species probably inhibit each other's reactivity. Herein, we have synthesized a novel Mnt-based multifunctional adsorbent (HFO-AZ16Mnt) via intercalation of zwitterionic surfactant (Z16), acid activation by chloric acid, and introduction of hydrated ferric oxides (HFOs). The acid activation can lead to formation of porous nanosilica, which serves as the new active sites for supporting HFO nanoparticles. Employing tetrachloroferrate (FeCl

Identifiants

pubmed: 33610995
pii: S0048-9697(21)00040-1
doi: 10.1016/j.scitotenv.2021.144974
pii:
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

144974

Informations de copyright

Copyright © 2021 Elsevier B.V. All rights reserved.

Déclaration de conflit d'intérêts

Declaration of competing interest The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper.

Auteurs

Yixuan Yang (Y)

CAS Key Laboratory of Mineralogy and Metallogeny/Guangdong Provincial Key Laboratory of Mineral Physics and Materials, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China; CAS Center for Excellence in Deep Earth Science, Guangzhou, 510640, China; University of Chinese Academy of Sciences, Beijing 100049, China; Institutions of Earth Science, Chinese Academy of Sciences, Beijing 100029, China.

Runliang Zhu (R)

CAS Key Laboratory of Mineralogy and Metallogeny/Guangdong Provincial Key Laboratory of Mineral Physics and Materials, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China; CAS Center for Excellence in Deep Earth Science, Guangzhou, 510640, China; University of Chinese Academy of Sciences, Beijing 100049, China; Institutions of Earth Science, Chinese Academy of Sciences, Beijing 100029, China.

Qingze Chen (Q)

CAS Key Laboratory of Mineralogy and Metallogeny/Guangdong Provincial Key Laboratory of Mineral Physics and Materials, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China; CAS Center for Excellence in Deep Earth Science, Guangzhou, 510640, China; University of Chinese Academy of Sciences, Beijing 100049, China; Institutions of Earth Science, Chinese Academy of Sciences, Beijing 100029, China. Electronic address: chenqingze@gig.ac.cn.

Jieqi Xing (J)

CAS Key Laboratory of Mineralogy and Metallogeny/Guangdong Provincial Key Laboratory of Mineral Physics and Materials, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China; CAS Center for Excellence in Deep Earth Science, Guangzhou, 510640, China; University of Chinese Academy of Sciences, Beijing 100049, China; Institutions of Earth Science, Chinese Academy of Sciences, Beijing 100029, China.

Lingya Ma (L)

CAS Key Laboratory of Mineralogy and Metallogeny/Guangdong Provincial Key Laboratory of Mineral Physics and Materials, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China; CAS Center for Excellence in Deep Earth Science, Guangzhou, 510640, China; University of Chinese Academy of Sciences, Beijing 100049, China; Institutions of Earth Science, Chinese Academy of Sciences, Beijing 100029, China.

Qiuzhi He (Q)

CAS Key Laboratory of Mineralogy and Metallogeny/Guangdong Provincial Key Laboratory of Mineral Physics and Materials, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China; CAS Center for Excellence in Deep Earth Science, Guangzhou, 510640, China; University of Chinese Academy of Sciences, Beijing 100049, China; Institutions of Earth Science, Chinese Academy of Sciences, Beijing 100029, China.

Jian Fan (J)

Technology Innovation Center of Ecological Monitoring & Restoration Project on Land (arable), MNR Geological Survey of Jiangsu Province, Nanjing 210018, China.

Yunfei Xi (Y)

School of Earth and Atmospheric Sciences & Institute for Future Environments, Queensland University of Technology, Brisbane, QLD 4001, Australia. Electronic address: y.xi@qut.edu.au.

Jianxi Zhu (J)

CAS Key Laboratory of Mineralogy and Metallogeny/Guangdong Provincial Key Laboratory of Mineral Physics and Materials, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China; CAS Center for Excellence in Deep Earth Science, Guangzhou, 510640, China; University of Chinese Academy of Sciences, Beijing 100049, China; Institutions of Earth Science, Chinese Academy of Sciences, Beijing 100029, China.

Hongping He (H)

CAS Key Laboratory of Mineralogy and Metallogeny/Guangdong Provincial Key Laboratory of Mineral Physics and Materials, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China; CAS Center for Excellence in Deep Earth Science, Guangzhou, 510640, China; University of Chinese Academy of Sciences, Beijing 100049, China; Institutions of Earth Science, Chinese Academy of Sciences, Beijing 100029, China.

Classifications MeSH