Cytotoxicity, Retention, and Anti-inflammatory Effects of a CeO


Journal

ACS pharmacology & translational science
ISSN: 2575-9108
Titre abrégé: ACS Pharmacol Transl Sci
Pays: United States
ID NLM: 101721411

Informations de publication

Date de publication:
12 Feb 2021
Historique:
received: 15 10 2020
entrez: 22 2 2021
pubmed: 23 2 2021
medline: 23 2 2021
Statut: epublish

Résumé

Both cerium oxide (CeOx) nanoparticles and mefenamic acid (MFA) are known anti-inflammatory agents with hepatoprotective properties and are therefore prescribed for one of the major diseases in the world, nonalcoholic fatty liver disease (NAFLD). To study the potential cytotoxicity and anti-inflammatory effects as well as drug retention of a potential therapeutic CeOx/MFA supramolecular complex, a well-standardized hepatic (HepG2) spheroid model was used. Results showed that the highest cytotoxicity for the CeOx/MFA supramolecular complex was found at 50 μg/mL, while effective doses of 0.1 and 1 μg/mL yielded a significant decrease of TNF-α and IL-8 secretion. Time-resolved analysis of HepG2 spheroids revealed a spatiotemporal distribution of the supramolecular complex and limited clearance from the internal microtissue over a period of 8 days in cultivation. In summary, our results point at rapid uptake, distribution, and biostability of the supramolecular complex within the HepG2 liver spheroid model as well as a significant anti-inflammatory response at noncytotoxic levels.

Identifiants

pubmed: 33615164
doi: 10.1021/acsptsci.0c00170
pmc: PMC7887746
doi:

Types de publication

Journal Article

Langues

eng

Pagination

101-106

Informations de copyright

© 2020 American Chemical Society.

Déclaration de conflit d'intérêts

The authors declare the following competing financial interest(s): Work in this paper was partially supported by funding from Farmak JSC who also produced the supramolecular complex in cooperation with the Institute for Scintillation Materials. All experiments were performed by the Technical University of Vienna in cooperation with SAICO Biosystems.

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Auteurs

Christoph Eilenberger (C)

Institute of Chemical Technologies and Analytics and Institute of Applied Synthetic Chemistry, Faculty of Technical Chemistry, Vienna University of Technology, Getreidemarkt 9, 1060 Vienna, Austria.
SAICO Biosystems KG, Gumpendorferstraße 5/8, 1060 Vienna, Austria.
Austrian Cluster for Tissue Regeneration, Donaueschingenstraße 13, 1200 Vienna, Austria.

Florian Selinger (F)

Institute of Chemical Technologies and Analytics and Institute of Applied Synthetic Chemistry, Faculty of Technical Chemistry, Vienna University of Technology, Getreidemarkt 9, 1060 Vienna, Austria.
SAICO Biosystems KG, Gumpendorferstraße 5/8, 1060 Vienna, Austria.
Austrian Cluster for Tissue Regeneration, Donaueschingenstraße 13, 1200 Vienna, Austria.

Mario Rothbauer (M)

Institute of Chemical Technologies and Analytics and Institute of Applied Synthetic Chemistry, Faculty of Technical Chemistry, Vienna University of Technology, Getreidemarkt 9, 1060 Vienna, Austria.
SAICO Biosystems KG, Gumpendorferstraße 5/8, 1060 Vienna, Austria.
Austrian Cluster for Tissue Regeneration, Donaueschingenstraße 13, 1200 Vienna, Austria.
Medical University of Vienna, Department of Orthopedics and Trauma Surgery, Karl Chiari Lab for Orthopaedic Biology, Währingergürtel 18-19, 1090 Vienna, Austria.

Yiji Lin (Y)

Institute of Chemical Technologies and Analytics and Institute of Applied Synthetic Chemistry, Faculty of Technical Chemistry, Vienna University of Technology, Getreidemarkt 9, 1060 Vienna, Austria.

Andreas Limbeck (A)

Institute of Chemical Technologies and Analytics and Institute of Applied Synthetic Chemistry, Faculty of Technical Chemistry, Vienna University of Technology, Getreidemarkt 9, 1060 Vienna, Austria.

Barbara Schädl (B)

Ludwig-Boltzmann-Institute for Experimental and Clinical Traumatology, Donaueschingenstraße 13, 1200 Vienna, Austria.
Austrian Cluster for Tissue Regeneration, Donaueschingenstraße 13, 1200 Vienna, Austria.

Johannes Grillari (J)

Ludwig-Boltzmann-Institute for Experimental and Clinical Traumatology, Donaueschingenstraße 13, 1200 Vienna, Austria.
Austrian Cluster for Tissue Regeneration, Donaueschingenstraße 13, 1200 Vienna, Austria.
University of Natural Resources and Life Sciences, Dept. of Biotechnology, Institute for Molecular Biotechnology, Muthgasse 18, 1190 Vienna, Austria.

Nataliya S Kavok (NS)

Institute for Scintillation Materials, STC "Institute for Single Crystals", 60 Science Avenue, 61001 Kharkiv, Ukraine.

Vladimir K Klochkov (VK)

Institute for Scintillation Materials, STC "Institute for Single Crystals", 60 Science Avenue, 61001 Kharkiv, Ukraine.

Yuri V Malyukin (YV)

Institute for Scintillation Materials, STC "Institute for Single Crystals", 60 Science Avenue, 61001 Kharkiv, Ukraine.

Victor Margitich (V)

Farmak JSC, 63, Kyrylivska Street, Kiev 04080, Ukraine.

Peter Ertl (P)

Institute of Chemical Technologies and Analytics and Institute of Applied Synthetic Chemistry, Faculty of Technical Chemistry, Vienna University of Technology, Getreidemarkt 9, 1060 Vienna, Austria.
SAICO Biosystems KG, Gumpendorferstraße 5/8, 1060 Vienna, Austria.
Austrian Cluster for Tissue Regeneration, Donaueschingenstraße 13, 1200 Vienna, Austria.

Classifications MeSH