Analysis of External and Internal Disorder to Understand Band-Like Transport in n-Type Organic Semiconductors.
charge transport
disorder
field-effect transistors
organic semiconductors
phonons
Journal
Advanced materials (Deerfield Beach, Fla.)
ISSN: 1521-4095
Titre abrégé: Adv Mater
Pays: Germany
ID NLM: 9885358
Informations de publication
Date de publication:
Apr 2021
Apr 2021
Historique:
revised:
18
01
2021
received:
19
11
2020
pubmed:
26
2
2021
medline:
26
2
2021
entrez:
25
2
2021
Statut:
ppublish
Résumé
Charge transport in organic semiconductors is notoriously extremely sensitive to the presence of disorder, both internal and external (i.e., related to interactions with the dielectric layer), especially for n-type materials. Internal dynamic disorder stems from large thermal fluctuations both in intermolecular transfer integrals and (molecular) site energies in weakly interacting van der Waals solids and sources transient localization of the charge carriers. The molecular vibrations that drive transient localization typically operate at low-frequency (<a-few-hundred cm
Identifiants
pubmed: 33629772
doi: 10.1002/adma.202007870
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
e2007870Subventions
Organisme : Natural Sciences and Engineering Research Council of Canada
Organisme : Fonds de Recherche du Québec - Nature et Technologies
Organisme : ERC
ID : GA-257305
Organisme : UHMob
ID : GA- 811284
Organisme : Labex projects CSC
ID : ANR-10-LABX-0026 CSC
Organisme : NIE
ID : ANR-11-LABX-0058 NIE
Organisme : Investissement d'Avenir program
ID : ANR-10-IDEX-0002-02
Organisme : International Center for Frontier Research in Chemistry
Organisme : Engineering and Physical Sciences Research Council
ID : EP/P00928X/1
Organisme : European Commission
Organisme : Région Wallonne
Organisme : Consortium des Équipements de Calcul Intensif
Organisme : Fonds National de la Recherche Scientifique
ID : 2.5020.11
Organisme : Fédération Wallonie-Bruxelles
Organisme : Walloon Region
ID : 1117545
Organisme : Horizon 2020
ID : 646176
Organisme : Marie Curie
ID : GA No. 813863
Pays : United Kingdom
Informations de copyright
© 2021 Wiley-VCH GmbH.
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