Effect of electrolyte flow on a gas evolution electrode.


Journal

Scientific reports
ISSN: 2045-2322
Titre abrégé: Sci Rep
Pays: England
ID NLM: 101563288

Informations de publication

Date de publication:
25 Feb 2021
Historique:
received: 27 10 2020
accepted: 15 01 2021
entrez: 26 2 2021
pubmed: 27 2 2021
medline: 27 2 2021
Statut: epublish

Résumé

In this study, the effect of flow of the electrolyte on an electrolysis cell and a zinc cell is investigated. The gain of energy brought by the flow is discussed and compared to the viscous losses in the cells. We point out that the balance between the gained electrical power and the viscous loss power is positive only if the hydrodynamic resistance of the circuit is correctly designed and further comment on the economical viability of the whole process. A model of the studied phenomena is proposed in the last section. This analytical model captures the dynamics of the process, gives the optimal flowing conditions and the limits of the energetical rentability of the process. This study shows that the use of flowing electrolyte in zinc-air batteries can be energetically profitable with the appropriate flowing conditions.

Identifiants

pubmed: 33633235
doi: 10.1038/s41598-021-84084-1
pii: 10.1038/s41598-021-84084-1
pmc: PMC7907386
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

4677

Références

Adv Mater. 2017 Feb;29(7):
pubmed: 27892635
Chem Sci. 2019 Sep 10;10(40):9165-9181
pubmed: 32015799

Auteurs

Soufiane Abdelghani-Idrissi (S)

ESPCI Paris, PSL Research University, MIE-CBI, CNRS UMR 8231, 10, Rue Vauquelin, 75231, Paris Cedex 05, France.

Nicolas Dubouis (N)

Chimie du Solide et de l'Energie, Collège de France, UMR 8260, 75231, Paris Cedex 05, France.
Sorbonne Université, Paris, France.
Réseau sur le Stockage Electrochimique de l'Energie (RS2E), CNRS FR 3459, 75005 80039 Cedex, Amiens, France.

Alexis Grimaud (A)

Chimie du Solide et de l'Energie, Collège de France, UMR 8260, 75231, Paris Cedex 05, France.
Sorbonne Université, Paris, France.
Réseau sur le Stockage Electrochimique de l'Energie (RS2E), CNRS FR 3459, 75005 80039 Cedex, Amiens, France.

Philippe Stevens (P)

Réseau sur le Stockage Electrochimique de l'Energie (RS2E), CNRS FR 3459, 75005 80039 Cedex, Amiens, France.
EDF R&D, EDF Lab Renardières, Département LME, 7 avenue des Renardières, 77818, Moret-sur-Loing cedex, France.

Gwenaëlle Toussaint (G)

Réseau sur le Stockage Electrochimique de l'Energie (RS2E), CNRS FR 3459, 75005 80039 Cedex, Amiens, France.
EDF R&D, EDF Lab Renardières, Département LME, 7 avenue des Renardières, 77818, Moret-sur-Loing cedex, France.

Annie Colin (A)

ESPCI Paris, PSL Research University, MIE-CBI, CNRS UMR 8231, 10, Rue Vauquelin, 75231, Paris Cedex 05, France. annie.colin@espci.fr.

Classifications MeSH