Colorful Efficient Moiré-Perovskite Solar Cells.
DVD disc
light diffraction
micro-nano imprinting
moiré interference structure
perovskite solar cells
Journal
Advanced materials (Deerfield Beach, Fla.)
ISSN: 1521-4095
Titre abrégé: Adv Mater
Pays: Germany
ID NLM: 9885358
Informations de publication
Date de publication:
Apr 2021
Apr 2021
Historique:
revised:
11
01
2021
received:
01
12
2020
pubmed:
7
3
2021
medline:
7
3
2021
entrez:
6
3
2021
Statut:
ppublish
Résumé
Light harvesting is crucial for thin-film solar cells. To substantially reduce optical loss in perovskite solar cells (PSCs), hierarchical light-trapping nano-architectures enable absorption enhancement to exceed the conventional upper limit and have great potential for achieving state-of-the art optoelectronic performances. However, it remains a great challenge to design and fabricate a superior hierarchical light-trapping nano-architecture, which exhibits extraordinary light-harvesting ability and simultaneously avoids deteriorating the electrical performance of PSCs. Herein, colorful efficient moiré-PSCs are designed and fabricated incorporating moiré interference structures by the imprinting method with the aid of a commercial DVD disc. It is experimentally and theoretically demonstrated that the light harvesting ability of the moiré interference structure can be well manipulated through changing the rotation angle (0°-90°). The boosted short-circuit current is credited to augment light diffraction channels, leading to elongated optical paths, and fold sunlight into the perovskite layer. Moreover, the imprinting process suppresses the trap sites and voids at the active-layer interfaces with eliminated hysteresis. The moiré-PSC with an optimized 30° rotation angle achieves the best enhancement of light harvesting (28.5% higher than the pristine), resulting in efficiencies over 20.17% (MAPbI
Identifiants
pubmed: 33675259
doi: 10.1002/adma.202008091
doi:
Types de publication
Journal Article
Review
Langues
eng
Sous-ensembles de citation
IM
Pagination
e2008091Subventions
Organisme : National Natural Science Foundation of China
ID : 52003273
Organisme : National Natural Science Foundation of China
ID : 22073107
Organisme : National Natural Science Foundation of China
ID : 21522308
Organisme : National Natural Science Foundation of China
ID : 51573192
Organisme : National Natural Science Foundation of China
ID : 51773206
Organisme : National Natural Science Foundation of China
ID : 91963212
Organisme : National Natural Science Foundation of China
ID : 61975177
Organisme : Beijing Natural Science Foundation
ID : 2194093
Organisme : Bureau of International Cooperation, Chinese Academy of Sciences
ID : GJHZ201948
Organisme : K.C. Wong Education Foundation, National Key R&D Program of China
ID : 2018YFA0208501
Organisme : Beijing National Laboratory for Molecular Sciences
ID : BNLMS- CXXM-202005
Informations de copyright
© 2021 Wiley-VCH GmbH.
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