Mobility of organic compounds in a soft clay-rich rock (Tégulines clay, France).

Absorption Adsorption Anion exclusion Clay rock Diffusion Organic compound

Journal

Chemosphere
ISSN: 1879-1298
Titre abrégé: Chemosphere
Pays: England
ID NLM: 0320657

Informations de publication

Date de publication:
Jul 2021
Historique:
received: 12 12 2020
revised: 15 02 2021
accepted: 19 02 2021
pubmed: 8 3 2021
medline: 14 5 2021
entrez: 7 3 2021
Statut: ppublish

Résumé

The migration of organic compounds in soils is a major concern in several environmental issues. Contaminants display distinct behaviours as regards to their specific affinities towards soils constituents. The retention mechanism of hydrophobic compounds by natural organic matter is well known. The retention of ionizable compounds is mainly related to oxides and clay minerals, even if less documented in reductive media. In this work, we investigated the migration of organic compounds in a soft clay-rich sedimentary rock (Tégulines clay, France). The aim was to determine the relative contributions of natural sorbents on retention, and eventual correlations with solutes properties. Both hydrophobic compounds (toluene, benzene, naphthalene) and hydrophilic species (adipate, oxalate, ortho-phthalate, benzoate) were investigated, using batch and diffusion experiments. The retention of neutral aromatic compounds correlates with their lipophilicity (log P

Identifiants

pubmed: 33677271
pii: S0045-6535(21)00517-8
doi: 10.1016/j.chemosphere.2021.130048
pii:
doi:

Substances chimiques

Aluminum Silicates 0
Organic Chemicals 0
Soil 0
Clay T1FAD4SS2M

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

130048

Informations de copyright

Copyright © 2021 Elsevier Ltd. All rights reserved.

Déclaration de conflit d'intérêts

Declaration of competing interest The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper.

Auteurs

Ning Guo (N)

Université Paris-Saclay, CEA, Service d'Étude du Comportement des Radionucléides, 91191, Gif-sur-Yvette, France.

Zoé Disdier (Z)

Université Paris-Saclay, CEA, Service d'Étude du Comportement des Radionucléides, 91191, Gif-sur-Yvette, France.

Émilie Thory (É)

Université Paris-Saclay, CEA, Service d'Étude du Comportement des Radionucléides, 91191, Gif-sur-Yvette, France.

Jean-Charles Robinet (JC)

Andra, R&D Division, Parc de la Croix Blanche, 92298, Châtenay-Malabry, France.

Romain V H Dagnelie (RVH)

Université Paris-Saclay, CEA, Service d'Étude du Comportement des Radionucléides, 91191, Gif-sur-Yvette, France. Electronic address: romain.dagnelie@cea.fr.

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Classifications MeSH