Tunable s-SNOM for Nanoscale Infrared Optical Measurement of Electronic Properties of Bilayer Graphene.


Journal

ACS photonics
ISSN: 2330-4022
Titre abrégé: ACS Photonics
Pays: United States
ID NLM: 101634366

Informations de publication

Date de publication:
17 Feb 2021
Historique:
received: 16 09 2020
entrez: 25 3 2021
pubmed: 26 3 2021
medline: 26 3 2021
Statut: ppublish

Résumé

Here we directly probe the electronic properties of bilayer graphene using s-SNOM measurements with a broadly tunable laser source over the energy range from 0.3 to 0.54 eV. We tune an OPO/OPA system around the interband resonance of Bernal stacked bilayer graphene (BLG) and extract amplitude and phase of the scattered light. This enables us to retrieve and reconstruct the complex optical conductivity resonance in BLG around 0.39 eV with nanoscale resolution. Our technique opens the door toward nanoscopic noncontact measurements of the electronic properties in complex hybrid 2D and van der Waals material systems, where scanning tunneling spectroscopy cannot access the decisive layers.

Identifiants

pubmed: 33763503
doi: 10.1021/acsphotonics.0c01442
pmc: PMC7976599
doi:

Types de publication

Journal Article

Langues

eng

Pagination

418-423

Informations de copyright

© 2021 American Chemical Society.

Déclaration de conflit d'intérêts

The authors declare the following competing financial interest(s): H. Linnenbank, T. Steinle, and H. Giessen are co-founders of SI Stuttgart Instruments GmbH, a company producing the OPO/OPA laser system such as the one used in this study. The other authors declare no conflict of interests.

Références

Nature. 2019 Sep;573(7772):91-95
pubmed: 31365921
Nano Lett. 2012 Aug 8;12(8):3973-8
pubmed: 22703339
Phys Rev Lett. 2011 Jan 28;106(4):046401
pubmed: 21405342
Nature. 2012 Jul 5;487(7405):77-81
pubmed: 22722861
Nat Mater. 2015 Apr;14(4):421-5
pubmed: 25532073
Nano Lett. 2017 Nov 8;17(11):7080-7085
pubmed: 28967761
Phys Rev Lett. 2008 Nov 7;101(19):196405
pubmed: 19113291
ACS Nano. 2015 Jul 28;9(7):6765-73
pubmed: 26050795
Nature. 2019 Aug;572(7767):101-105
pubmed: 31367031
Nat Mater. 2016 Aug;15(8):840-4
pubmed: 27240109
Nat Commun. 2015 Jun 26;6:7507
pubmed: 26112474
Science. 2014 Mar 7;343(6175):1125-9
pubmed: 24604197
Nature. 2009 Jun 11;459(7248):820-3
pubmed: 19516337
Proc Natl Acad Sci U S A. 2010 Aug 24;107(34):14999-5004
pubmed: 20696939
Nature. 2018 Apr 5;556(7699):43-50
pubmed: 29512651
Nature. 2015 Apr 30;520(7549):650-5
pubmed: 25901686
J Phys Condens Matter. 2013 May 29;25(21):215301
pubmed: 23628895
Opt Express. 2012 Jun 4;20(12):13173-88
pubmed: 22714345
Opt Express. 2007 Jul 9;15(14):8550-65
pubmed: 19547189
Nature. 2019 Aug;572(7767):95-100
pubmed: 31367030
Phys Rev Lett. 2016 Aug 19;117(8):086801
pubmed: 27588873
Science. 2018 Dec 7;362(6419):1153-1156
pubmed: 30523109
Nature. 2012 Jul 5;487(7405):82-5
pubmed: 22722866
Nanoscale. 2017 Mar 23;9(12):4191-4195
pubmed: 28287222

Auteurs

Konstantin G Wirth (KG)

I. Institute of Physics (IA), RWTH Aachen University, 52074 Aachen, Germany.

Heiko Linnenbank (H)

4th Physics Institute and Research Center SCoPE, University of Stuttgart, 70569 Stuttgart, Germany.
SI Stuttgart Instruments GmbH, 70771 Leinfelden-Echterdingen, Germany.

Tobias Steinle (T)

4th Physics Institute and Research Center SCoPE, University of Stuttgart, 70569 Stuttgart, Germany.
SI Stuttgart Instruments GmbH, 70771 Leinfelden-Echterdingen, Germany.

Luca Banszerus (L)

2nd Institute of Physics (IIA), RWTH Aachen University, 52074 Aachen, Germany.

Eike Icking (E)

2nd Institute of Physics (IIA), RWTH Aachen University, 52074 Aachen, Germany.

Christoph Stampfer (C)

2nd Institute of Physics (IIA), RWTH Aachen University, 52074 Aachen, Germany.
Jülich Aachen Research Alliance - Fundamentals of Future Information Technology (JARA-FIT), 52074 Aachen, Germany.

Harald Giessen (H)

4th Physics Institute and Research Center SCoPE, University of Stuttgart, 70569 Stuttgart, Germany.
SI Stuttgart Instruments GmbH, 70771 Leinfelden-Echterdingen, Germany.

Thomas Taubner (T)

I. Institute of Physics (IA), RWTH Aachen University, 52074 Aachen, Germany.
Jülich Aachen Research Alliance - Fundamentals of Future Information Technology (JARA-FIT), 52074 Aachen, Germany.

Classifications MeSH