3-Carboxylic Acid and Formyl-Derived Coumarins as Photoinitiators in Photo-Oxidation or Photo-Reduction Processes for Photopolymerization upon Visible Light: Photocomposite Synthesis and 3D Printing Applications.

LED coumarin direct laser write free radical polymerization photocomposites

Journal

Molecules (Basel, Switzerland)
ISSN: 1420-3049
Titre abrégé: Molecules
Pays: Switzerland
ID NLM: 100964009

Informations de publication

Date de publication:
21 Mar 2021
Historique:
received: 22 02 2021
revised: 13 03 2021
accepted: 18 03 2021
entrez: 3 4 2021
pubmed: 4 4 2021
medline: 4 4 2021
Statut: epublish

Résumé

In this paper, nine organic compounds based on the coumarin scaffold and different substituents were synthesized and used as high-performance photoinitiators for free radical photopolymerization (FRP) of meth(acrylate) functions under visible light irradiation using LED at 405 nm. In fact, these compounds showed a very high initiation capacity and very good polymerization profiles (both high rate of polymerization (Rp) and final conversion (FC)) using two and three-component photoinitiating systems based on coum/iodonium salt (0.1%/1%

Identifiants

pubmed: 33800978
pii: molecules26061753
doi: 10.3390/molecules26061753
pmc: PMC8003961
pii:
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Subventions

Organisme : Aix-Marseille Université
ID : permanent fundings
Organisme : Agence Nationale de la Recherche
ID : ANR-17-CE08-0054 VISICAT project
Organisme : Centre National de la Recherche Scientifique
ID : permanent fundings
Organisme : Université de Haute Alsace
ID : Permanent fundings

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Auteurs

Mahmoud Rahal (M)

CNRS, IS2M UMR 7361, Université de Haute-Alsace, F-68100 Mulhouse, France.
Université de Strasbourg, 67081 Strasbourg, France.
Laboratory of Materials, Catalysis, Environment and Analytical Methods (MCEMA) and LEADDER Laboratory, Faculty of Sciences, Doctoral School of Sciences and Technology (EDST), Lebanese University, Beirut 6573-14, Lebanon.

Bernadette Graff (B)

CNRS, IS2M UMR 7361, Université de Haute-Alsace, F-68100 Mulhouse, France.
Université de Strasbourg, 67081 Strasbourg, France.

Joumana Toufaily (J)

Laboratory of Materials, Catalysis, Environment and Analytical Methods (MCEMA) and LEADDER Laboratory, Faculty of Sciences, Doctoral School of Sciences and Technology (EDST), Lebanese University, Beirut 6573-14, Lebanon.

Tayssir Hamieh (T)

Laboratory of Materials, Catalysis, Environment and Analytical Methods (MCEMA) and LEADDER Laboratory, Faculty of Sciences, Doctoral School of Sciences and Technology (EDST), Lebanese University, Beirut 6573-14, Lebanon.
SATIE-IFSTTAR, Université Gustave Eiffel, Campus de Marne-La-Vallée, 25, allée des Marronniers, F-78000 Versailles, France.

Guillaume Noirbent (G)

CNRS, ICR UMR 7273, Aix Marseille Université, F-13397 Marseille, France.

Didier Gigmes (D)

CNRS, ICR UMR 7273, Aix Marseille Université, F-13397 Marseille, France.

Frédéric Dumur (F)

CNRS, ICR UMR 7273, Aix Marseille Université, F-13397 Marseille, France.

Jacques Lalevée (J)

CNRS, IS2M UMR 7361, Université de Haute-Alsace, F-68100 Mulhouse, France.
Université de Strasbourg, 67081 Strasbourg, France.

Classifications MeSH