Intrinsic Electrocatalytic Activity for Oxygen Evolution of Crystalline 3d-Transition Metal Layered Double Hydroxides.

electrochemical surface area hydrothermal synthesis layered double hydroxides oxygen evolution reaction water splitting

Journal

Angewandte Chemie (International ed. in English)
ISSN: 1521-3773
Titre abrégé: Angew Chem Int Ed Engl
Pays: Germany
ID NLM: 0370543

Informations de publication

Date de publication:
21 Jun 2021
Historique:
received: 14 01 2021
pubmed: 13 4 2021
medline: 13 4 2021
entrez: 12 4 2021
Statut: ppublish

Résumé

Layered double hydroxides (LDHs) are among the most active and studied catalysts for the oxygen evolution reaction (OER) in alkaline electrolytes. However, previous studies have generally either focused on a small number of LDHs, applied synthetic routes with limited structural control, or used non-intrinsic activity metrics, thus hampering the construction of consistent structure-activity-relations. Herein, by employing new individually developed synthesis strategies with atomic structural control, we obtained a broad series of crystalline α-M

Identifiants

pubmed: 33844879
doi: 10.1002/anie.202100631
pmc: PMC8252729
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

14446-14457

Subventions

Organisme : Deutsche Forschungsgemeinschaft
ID : STR 596/12-1
Organisme : Frontier Science Key Project of the Chinese Academy of Sciences
ID : QYZDJSSW-SLH054
Organisme : Intramural NIH HHS
ID : Z01 SC010379
Pays : United States
Organisme : National Key R&D Program of China
ID : 2018YFA0208603
Organisme : Office of Science, Office of Basic Energy Sciences, Chemical, Biological, and Geosciences Division
ID : DE-SC0010379
Organisme : ECS Toyota Young Investigator Fellowship
Organisme : the Bundesministerium für Wirtschaft (BMWi)
ID : 03EIV041F (MethQuest/MethFuel)
Organisme : the Bundesministerium für Bildung und Forschung (BMBF)
ID : 03SF0611A (H2-Meer) and 03SF0613D (AEMready)
Organisme : K. C. Wong Education
ID : GJTD-2020-15

Informations de copyright

© 2021 The Authors. Angewandte Chemie International Edition published by Wiley-VCH GmbH.

Références

Science. 2008 Aug 22;321(5892):1072-5
pubmed: 18669820
Nat Chem. 2014 Apr;6(4):362-7
pubmed: 24651205
J Phys Chem Lett. 2015 Sep 17;6(18):3737-42
pubmed: 26722749
Nat Mater. 2012 May 06;11(6):550-7
pubmed: 22561903
Angew Chem Int Ed Engl. 2020 May 18;59(21):8072-8077
pubmed: 32078226
Nat Commun. 2020 May 20;11(1):2522
pubmed: 32433529
Nat Commun. 2015 Oct 12;6:8625
pubmed: 26456525
J Am Chem Soc. 2014 May 7;136(18):6744-53
pubmed: 24779732
Chemphyschem. 2010 Jun 21;11(9):1854-7
pubmed: 20473978
J Am Chem Soc. 2012 Oct 17;134(41):17253-61
pubmed: 22991896
J Am Chem Soc. 2013 Nov 13;135(45):16977-87
pubmed: 24171402
J Am Chem Soc. 2014 Nov 26;136(47):16481-4
pubmed: 25380057
Angew Chem Int Ed Engl. 2021 Jun 21;60(26):14446-14457
pubmed: 33844879
Nat Commun. 2014 Jul 17;5:4477
pubmed: 25030209
Science. 2019 Feb 22;363(6429):870-874
pubmed: 30792302
Proc Natl Acad Sci U S A. 2018 Jun 5;115(23):5872-5877
pubmed: 29784794
J Am Chem Soc. 2015 Mar 18;137(10):3638-48
pubmed: 25700234
J Am Chem Soc. 2015 Dec 9;137(48):15090-3
pubmed: 26601790
J Am Chem Soc. 2018 Jun 6;140(22):6745-6748
pubmed: 29749225
Nature. 2020 Nov;587(7834):408-413
pubmed: 33208960
J Am Chem Soc. 2015 Jan 28;137(3):1305-13
pubmed: 25562406
Science. 2011 Dec 9;334(6061):1383-5
pubmed: 22033519
Science. 2016 Sep 2;353(6303):1011-1014
pubmed: 27701108

Auteurs

Fabio Dionigi (F)

The Electrochemical Energy, Catalysis, and Materials Science Laboratory, Department of Chemistry, Chemical Engineering Division, Technical University Berlin, Strasse des 17. Juni 124, 10623, Berlin, Germany.

Jing Zhu (J)

School of Chemistry and Materials Science, CAS Excellence Center for Nanoscience, Hefei National Laboratory for Physical Sciences at Microscale, University of Science and Technology of China, Hefei, 230026, Anhui, China.

Zhenhua Zeng (Z)

Davidson School of Chemical Engineering, Purdue University, West Lafayette, IN, 47907, USA.

Thomas Merzdorf (T)

The Electrochemical Energy, Catalysis, and Materials Science Laboratory, Department of Chemistry, Chemical Engineering Division, Technical University Berlin, Strasse des 17. Juni 124, 10623, Berlin, Germany.

Hannes Sarodnik (H)

The Electrochemical Energy, Catalysis, and Materials Science Laboratory, Department of Chemistry, Chemical Engineering Division, Technical University Berlin, Strasse des 17. Juni 124, 10623, Berlin, Germany.

Manuel Gliech (M)

The Electrochemical Energy, Catalysis, and Materials Science Laboratory, Department of Chemistry, Chemical Engineering Division, Technical University Berlin, Strasse des 17. Juni 124, 10623, Berlin, Germany.

Lujin Pan (L)

The Electrochemical Energy, Catalysis, and Materials Science Laboratory, Department of Chemistry, Chemical Engineering Division, Technical University Berlin, Strasse des 17. Juni 124, 10623, Berlin, Germany.

Wei-Xue Li (WX)

School of Chemistry and Materials Science, CAS Excellence Center for Nanoscience, Hefei National Laboratory for Physical Sciences at Microscale, University of Science and Technology of China, Hefei, 230026, Anhui, China.

Jeffrey Greeley (J)

Davidson School of Chemical Engineering, Purdue University, West Lafayette, IN, 47907, USA.

Peter Strasser (P)

The Electrochemical Energy, Catalysis, and Materials Science Laboratory, Department of Chemistry, Chemical Engineering Division, Technical University Berlin, Strasse des 17. Juni 124, 10623, Berlin, Germany.

Classifications MeSH