Global Phosphoproteomics Reveal CDK Suppression as a Vulnerability to KRas Addiction in Pancreatic Cancer.


Journal

Clinical cancer research : an official journal of the American Association for Cancer Research
ISSN: 1557-3265
Titre abrégé: Clin Cancer Res
Pays: United States
ID NLM: 9502500

Informations de publication

Date de publication:
15 07 2021
Historique:
received: 10 12 2020
revised: 27 02 2021
accepted: 16 04 2021
pubmed: 22 4 2021
medline: 1 4 2022
entrez: 21 4 2021
Statut: ppublish

Résumé

Among human cancers that harbor mutant (mt) KRas, some, but not all, are dependent on mt KRas. However, little is known about what drives KRas dependency. Global phosphoproteomics, screening of a chemical library of FDA drugs, and genome-wide CRISPR/Cas9 viability database analysis were used to identify vulnerabilities of KRas dependency. Global phosphoproteomics revealed that KRas dependency is driven by a cyclin-dependent kinase (CDK) network. CRISPR/Cas9 viability database analysis revealed that, in mt KRas-driven pancreatic cancer cells, knocking out the cell-cycle regulators CDK1 or CDK2 or the transcriptional regulators CDK7 or CDK9 was as effective as knocking out KRas. Furthermore, screening of a library of FDA drugs identified AT7519, a CDK1, 2, 7, and 9 inhibitor, as a potent inducer of apoptosis in mt KRas-dependent, but not in mt KRas-independent, human cancer cells. A link between CDK hyperactivation and mt KRas dependency was uncovered and pharmacologically exploited to abrogate mt KRas-driven pancreatic cancer in highly relevant models, warranting clinical investigations of AT7519 in patients with pancreatic cancer.

Identifiants

pubmed: 33879459
pii: 1078-0432.CCR-20-4781
doi: 10.1158/1078-0432.CCR-20-4781
pmc: PMC8493485
mid: NIHMS1697823
doi:

Substances chimiques

KRAS protein, human 0
Proteome 0
Cyclin-Dependent Kinases EC 2.7.11.22
Hras protein, mouse EC 3.6.5.2
Proto-Oncogene Proteins p21(ras) EC 3.6.5.2

Types de publication

Journal Article Research Support, N.I.H., Extramural Research Support, Non-U.S. Gov't

Langues

eng

Sous-ensembles de citation

IM

Pagination

4012-4024

Subventions

Organisme : NCI NIH HHS
ID : P30 CA076292
Pays : United States
Organisme : NCI NIH HHS
ID : R01 CA242003
Pays : United States
Organisme : NCI NIH HHS
ID : R35 CA197731
Pays : United States
Organisme : NCI NIH HHS
ID : U54 CA233444
Pays : United States

Informations de copyright

©2021 American Association for Cancer Research.

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Auteurs

Aslamuzzaman Kazi (A)

Department of Drug Discovery, H. Lee Moffitt Cancer Center and Research Institute, Tampa, Florida.

Liwei Chen (L)

Department of Drug Discovery, H. Lee Moffitt Cancer Center and Research Institute, Tampa, Florida.

Shengyan Xiang (S)

Department of Drug Discovery, H. Lee Moffitt Cancer Center and Research Institute, Tampa, Florida.

Rajanikanth Vangipurapu (R)

Department of Drug Discovery, H. Lee Moffitt Cancer Center and Research Institute, Tampa, Florida.

Hua Yang (H)

Department of Drug Discovery, H. Lee Moffitt Cancer Center and Research Institute, Tampa, Florida.

Francisca Beato (F)

Department of Gastrointestinal Oncology, H. Lee Moffitt Cancer Center and Research Institute, Tampa, Florida.

Bin Fang (B)

Proteomics and Metabolomics Core, H. Lee Moffitt Cancer Center and Research Institute, Tampa, Florida.

Terence M Williams (TM)

Department of Radiation Oncology, The Ohio State University, Columbus, Ohio.

Kazim Husain (K)

Department of Gastrointestinal Oncology, H. Lee Moffitt Cancer Center and Research Institute, Tampa, Florida.

Patrick Underwood (P)

Department of Surgery, University of Florida, Gainesville, Florida.

Jason B Fleming (JB)

Department of Gastrointestinal Oncology, H. Lee Moffitt Cancer Center and Research Institute, Tampa, Florida.

Mokenge Malafa (M)

Department of Gastrointestinal Oncology, H. Lee Moffitt Cancer Center and Research Institute, Tampa, Florida.

Eric A Welsh (EA)

Biostatistics and Bioinformatics Shared Resource, H. Lee Moffitt Cancer Center and Research Institute, Tampa, Florida.

John Koomen (J)

Molecular Oncology Department, H. Lee Moffitt Cancer Center and Research Institute, Tampa, Florida.

José Trevino (J)

Department of Surgery, University of Florida, Gainesville, Florida.

Saïd M Sebti (SM)

Department of Drug Discovery, H. Lee Moffitt Cancer Center and Research Institute, Tampa, Florida. said.sebti@vcuhealth.org.
Chemical Biology and Molecular Medicine Program, H. Lee Moffitt Cancer Center and Research Institute, Tampa, Florida.

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Classifications MeSH