Catalytic fast pyrolysis of waste mixed cloth for the production of value-added chemicals.

Aromatics Catalytic fast pyrolysis Levoglucosan Waste mixed cloth

Journal

Waste management (New York, N.Y.)
ISSN: 1879-2456
Titre abrégé: Waste Manag
Pays: United States
ID NLM: 9884362

Informations de publication

Date de publication:
15 May 2021
Historique:
received: 04 01 2021
revised: 23 03 2021
accepted: 14 04 2021
pubmed: 3 5 2021
medline: 26 5 2021
entrez: 2 5 2021
Statut: ppublish

Résumé

In the present study, catalytic fast pyrolysis of waste mixed cloth in an ex-situ method using hierarchical HZSM and commercial CaO was investigated. Pyrolysis of waste mixed cloth in a temperature range of 450 °C to 750 °C mainly allowed for the formation of levoglucosan without any catalysts. The utilization of HZSM with Brønsted/Lewis acid sites on micro- and mesoporous structures significantly contributed to monocyclic/dicyclic chemicals production, mainly referring to monoaromatics and naphthalene-based derivatives, especially in the case of high heating rates and catalyst usages. Furthermore, CaO revealed strong deoxygenation performance for the transformation of waste mixed cloth into low oxygen-containing chemicals, such as ketones, aliphatic hydrocarbons and aromatics. The present research thus highlights a feasible route for the catalytic upgrading of waste mixed cloth into some kinds of value-added chemicals.

Identifiants

pubmed: 33933871
pii: S0956-053X(21)00234-8
doi: 10.1016/j.wasman.2021.04.036
pii:
doi:

Substances chimiques

Biofuels 0
Hydrocarbons 0

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

141-146

Informations de copyright

Copyright © 2021 Elsevier Ltd. All rights reserved.

Déclaration de conflit d'intérêts

Declaration of Competing Interest The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper.

Auteurs

Jun Zhang (J)

Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences (CAS), Guangzhou 510640, PR China; Southern Marine Science and Engineering Guangdong Laboratory (Guangzhou), 511458, PR China; CAS Key Laboratory of Renewable Energy, Guangzhou 510640, PR China; Guangdong Provincial Key Laboratory of New and Renewable Energy Research and Development, Guangzhou 510640, PR China.

Jing Gu (J)

Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences (CAS), Guangzhou 510640, PR China; Southern Marine Science and Engineering Guangdong Laboratory (Guangzhou), 511458, PR China; CAS Key Laboratory of Renewable Energy, Guangzhou 510640, PR China; Guangdong Provincial Key Laboratory of New and Renewable Energy Research and Development, Guangzhou 510640, PR China.

Haoran Yuan (H)

Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences (CAS), Guangzhou 510640, PR China; Southern Marine Science and Engineering Guangdong Laboratory (Guangzhou), 511458, PR China; CAS Key Laboratory of Renewable Energy, Guangzhou 510640, PR China; Guangdong Provincial Key Laboratory of New and Renewable Energy Research and Development, Guangzhou 510640, PR China. Electronic address: yuanhr@ms.giec.ac.cn.

Yong Chen (Y)

Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences (CAS), Guangzhou 510640, PR China; Southern Marine Science and Engineering Guangdong Laboratory (Guangzhou), 511458, PR China; CAS Key Laboratory of Renewable Energy, Guangzhou 510640, PR China; Guangdong Provincial Key Laboratory of New and Renewable Energy Research and Development, Guangzhou 510640, PR China.

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