Creating heralded hyper-entangled photons using Rydberg atoms.


Journal

Light, science & applications
ISSN: 2047-7538
Titre abrégé: Light Sci Appl
Pays: England
ID NLM: 101610753

Informations de publication

Date de publication:
12 May 2021
Historique:
received: 03 10 2020
accepted: 18 04 2021
revised: 15 03 2021
entrez: 12 5 2021
pubmed: 13 5 2021
medline: 13 5 2021
Statut: epublish

Résumé

Entangled photon pairs are a fundamental component for testing the foundations of quantum mechanics, and for modern quantum technologies such as teleportation and secured communication. Current state-of-the-art sources are based on nonlinear processes that are limited in their efficiency and wavelength tunability. This motivates the exploration of physical mechanisms for entangled photon generation, with a special interest in mechanisms that can be heralded, preferably at telecommunications wavelengths. Here we present a mechanism for the generation of heralded entangled photons from Rydberg atom cavity quantum electrodynamics (cavity QED). We propose a scheme to demonstrate the mechanism and quantify its expected performance. The heralding of the process enables non-destructive detection of the photon pairs. The entangled photons are produced by exciting a rubidium atom to a Rydberg state, from where the atom decays via two-photon emission (TPE). A Rydberg blockade helps to excite a single Rydberg excitation while the input light field is more efficiently collectively absorbed by all the atoms. The TPE rate is significantly enhanced by a designed photonic cavity, whose many resonances also translate into high-dimensional entanglement. The resulting high-dimensionally entangled photons are entangled in more than one degree of freedom: in all of their spectral components, in addition to the polarization-forming a hyper-entangled state, which is particularly interesting in high information capacity quantum communication. We characterize the photon comb states by analyzing the Hong-Ou-Mandel interference and propose proof-of-concept experiments.

Identifiants

pubmed: 33976109
doi: 10.1038/s41377-021-00537-2
pii: 10.1038/s41377-021-00537-2
pmc: PMC8113235
doi:

Types de publication

Journal Article

Langues

eng

Pagination

100

Commentaires et corrections

Type : ErratumIn

Références

Browne, D. E. & Rudolph, T. Resource-efficient linear optical quantum computation. Phys. Rev. Lett. 95, 010501 (2005).
doi: 10.1103/PhysRevLett.95.010501
Walther, P. et al. Experimental one-way quantum computing. Nature 434, 169–176 (2005).
doi: 10.1038/nature03347
Reimer, C. et al. High-dimensional one-way quantum processing implemented on d-level cluster states. Nat. Phys. 15, 148–153 (2019).
doi: 10.1038/s41567-018-0347-x
Bennett, C. H. et al. Teleporting an unknown quantum state via dual classical and Einstein-Podolsky-Rosen channels. Phys. Rev. Lett. 70, 1895–1899 (1993).
doi: 10.1103/PhysRevLett.70.1895
Bouwmeester, D. et al. Experimental quantum teleportation. Nature 390, 575–579 (1997).
doi: 10.1038/37539
Ma, X. S. et al. Quantum teleportation over 143 kilometres using active feed-forward. Nature 489, 269–273 (2012).
doi: 10.1038/nature11472
Mattle, K. et al. Dense coding in experimental quantum communication. Phys. Rev. Lett. 76, 4656–4659 (1996).
doi: 10.1103/PhysRevLett.76.4656
Wang, C. Y. et al. Generation of hyper-entangled photons in a hot atomic vapor. Opt. Lett. 45, 1802–1805 (2020).
doi: 10.1364/OL.384567
Marino, A. M. et al. Tunable delay of Einstein–Podolsky–Rosen entanglement. Nature 457, 859–862 (2009).
doi: 10.1038/nature07751
Riebe, M. et al. Deterministic quantum teleportation with atoms. Nature 429, 734–737 (2004).
doi: 10.1038/nature02570
Edamatsu, K. et al. Generation of ultraviolet entangled photons in a semiconductor. Nature 431, 167–170 (2004).
doi: 10.1038/nature02838
Hayat, A., Ginzburg, P. & Orenstein, M. Measurement and model of the infrared two-photon emission spectrum of GaAs. Phys. Rev. Lett. 103, 023601 (2009).
doi: 10.1103/PhysRevLett.103.023601
Young, R. J. et al. Improved fidelity of triggered entangled photons from single quantum dots. New J. Phys. 8, 29 (2006).
doi: 10.1088/1367-2630/8/2/029
Togan, E. et al. Quantum entanglement between an optical photon and a solid-state spin qubit. Nature 466, 730–734 (2010).
doi: 10.1038/nature09256
Reimer, C. et al. Cross-polarized photon-pair generation and bi-chromatically pumped optical parametric oscillation on a chip. Nat. Commun. 6, 8236 (2015).
doi: 10.1038/ncomms9236
Li, X. Y. et al. All-fiber source of frequency- entangled photon pairs. Phys. Rev. A 79, 033817 (2009).
doi: 10.1103/PhysRevA.79.033817
Kwiat, P. G. et al. New high-intensity source of polarization-entangled photon pairs. Phys. Rev. Lett. 75, 4337–4341 (1995).
doi: 10.1103/PhysRevLett.75.4337
Clark, A. S. et al. Heralded single-photon source in a III–V photonic crystal. Opt. Lett. 38, 649–651 (2013).
doi: 10.1364/OL.38.000649
Jin, R. B. et al. Efficient generation of twin photons at telecom wavelengths with 2.5 GHz repetition-rate-tunable comb laser. Sci. Rep. 4, 7468 (2014).
doi: 10.1038/srep07468
Solntsev, A. S. & Sukhorukov, A. A. Path-entangled photon sources on nonlinear chips. Rev. n Phys. 2, 19–31 (2017).
doi: 10.1016/j.revip.2016.11.003
Rangarajan, R. et al. Engineering an ideal indistinguishable photon-pair source for optical quantum information processing. J. Mod. Opt. 58, 318–327 (2011).
doi: 10.1080/09500340.2010.529515
Guo, X. et al. Parametric down-conversion photon-pair source on a nanophotonic chip. Light: Sci. Appl. 6, e16249 (2017).
doi: 10.1038/lsa.2016.249
Śliwa, C. & Banaszek, K. Conditional preparation of maximal polarization entanglement. Phys. Rev. A 67, 030101(R) (2003).
doi: 10.1103/PhysRevA.67.030101
Pittman, T. B. et al. Heralded two-photon entanglement from probabilistic quantum logic operations on multiple parametric down-conversion sources. IEEE J. Sel. Top. Quantum Electron. 9, 1478–1482 (2003).
doi: 10.1109/JSTQE.2003.820916
Barz, S. et al. Heralded generation of entangled photon pairs. Nat. Photonics 4, 553–556 (2010).
doi: 10.1038/nphoton.2010.156
Diddams, S. A., Vahala, K. & Udem, T. Optical frequency combs: coherently uniting the electromagnetic spectrum. Science 369, eaay3676 (2020).
doi: 10.1126/science.aay3676
Keller, U. Optical frequency combs from ultrafast solid-state and semiconductor lasers. Proc. SPIE 11460, https://doi.org/10.1117/12.2572134 (2020).
https://github.com/sutapag/TPE-Rydberg (2020).
Steinlechner, F. et al. Distribution of high-dimensional entanglement via an intra-city free-space link. Nat. Commun. 8, 15971 (2017).
doi: 10.1038/ncomms15971
Cozzolino, D. et al. High-dimensional quantum communication: benefits, progress, and future challenges. Adv. Quantum Technol. 2, 1900038 (2019).
doi: 10.1002/qute.201900038
Kues, M. et al. On-chip generation of high-dimensional entangled quantum states and their coherent control. Nature 546, 622–626 (2017).
doi: 10.1038/nature22986
Barreiro, J. T., Wei, T. C. & Kwiat, P. G. Beating the channel capacity limit for linear photonic superdense coding. Nat. Phys. 4, 282–286 (2008).
doi: 10.1038/nphys919
Walborn, S. P. Breaking the communication barrier. Nat. Phys. 4, 268–269 (2008).
doi: 10.1038/nphys927
Hu, X. M. et al. Beating the channel capacity limit for superdense coding with entangled ququarts. Sci. Adv. 4, eaat9304 (2018).
doi: 10.1126/sciadv.aat9304
Xie, Z. D. et al. Harnessing high-dimensional hyperentanglement through a biphoton frequency comb. Nat. Photonics 9, 536–542 (2015).
doi: 10.1038/nphoton.2015.110
Hu, X. M. et al. Efficient generation of high-dimensional entanglement through multipath down-conversion. Phys. Rev. Lett. 125, 090503 (2020).
doi: 10.1103/PhysRevLett.125.090503
Roslund, J. et al. Wavelength-multiplexed quantum networks with ultrafast frequency combs. Nat. Photonics 8, 109–112 (2014).
doi: 10.1038/nphoton.2013.340
Bernhard, C. et al. Shaping frequency-entangled qudits. Phys. Rev. A 88, 032322 (2013).
doi: 10.1103/PhysRevA.88.032322
Steinlechner, F. et al. Distribution of high-dimensional entanglement via an intra-city free-space link. Nat. Commun. 8, 15971 (2017).
doi: 10.1038/ncomms15971
Hu, X. M. et al. Efficient distribution of high-dimensional entanglement through 11 km fiber. Optica 7, 738–743 (2020).
doi: 10.1364/OPTICA.388773
Wang, X. L. et al. Quantum teleportation of multiple degrees of freedom of a single photon. Nature 518, 516–519 (2015).
doi: 10.1038/nature14246
Erhard, M., Krenn, M. & Zeilinger, A. Advances in high-dimensional quantum entanglement. Nature Rev. Phys. 2, 365–381 (2020).
doi: 10.1038/s42254-020-0193-5
Sheng, Y. B. & Deng, F. G. Deterministic entanglement purification and complete nonlocal bell-state analysis with hyperentanglement. Phys. Rev. A 81, 032307 (2010).
doi: 10.1103/PhysRevA.81.032307
Gaëtan, A. et al. Observation of collective excitation of two individual atoms in the Rydberg blockade regime. Nat. Phys. 5, 115–118 (2009).
doi: 10.1038/nphys1183
Paris-Mandoki, A. et al. Free-space quantum electrodynamics with a single Rydberg superatom. Phys. Rev. X 7, 041010 (2017).
Jaksch, D. et al. Fast quantum gates for neutral atoms. Phys. Rev. Lett. 85, 2208–2211 (2000).
doi: 10.1103/PhysRevLett.85.2208
Lukin, M. D. et al. Dipole blockade and quantum information processing in mesoscopic atomic ensembles. Phys. Rev. Lett. 87, 037901 (2001).
doi: 10.1103/PhysRevLett.87.037901
Saffman, M., Walker, T. G. & Mølmer, K. Quantum information with Rydberg atoms. Rev. Mod. Phys. 82, 2313–2363 (2010).
doi: 10.1103/RevModPhys.82.2313
Guo, C. Y. et al. Optimized geometric quantum computation with a mesoscopic ensemble of Rydberg atoms. Phys. Rev. A 102, 042607 (2020).
doi: 10.1103/PhysRevA.102.042607
Su, S. L. et al. One-step implementation of the Rydberg-Rydberg-Interaction gate. Phys. Rev. A 93, 012306 (2016).
doi: 10.1103/PhysRevA.93.012306
Su, S. L. et al. Fast Rydberg antiblockade regime and its applications in quantum logic gates. Phys. Rev. A 95, 022319 (2017).
doi: 10.1103/PhysRevA.95.022319
Su, S. L. et al. One-step construction of the multiple-qubit Rydberg controlled-phase gate. Phys. Rev. A 98, 032306 (2018).
doi: 10.1103/PhysRevA.98.032306
Su, S. L. et al. Rydberg antiblockade regimes: dynamics and applications. EPL (Europhys. Lett. 131, 53001 (2020).
Rivera, N. et al. Shrinking light to allow forbidden transitions on the atomic scale. Science 353, 263–269 (2016).
doi: 10.1126/science.aaf6308
Rivera, N. et al. Making two-photon processes dominate one-photon processes using mid-IR phonon polaritons. Proc. Natl Acad. Sci. USA 114, 13607–13612 (2017).
doi: 10.1073/pnas.1713538114
Ripka, F. et al. A room-temperature single-photon source based on strongly interacting Rydberg atoms. Science 362, 446–449 (2018).
doi: 10.1126/science.aau1949
Göppert-Mayer, M. Elementary processes with two quantum transitions. Annal. Physik 18, 466–479 (2009).
doi: 10.1002/andp.200952107-804
Cresser, J. D. et al. Lifetime of excited atomic states. Phys. Rev. A 33, 1677–1682 (1986).
doi: 10.1103/PhysRevA.33.1677
Florescu, V. Two-photon emissionn in the 3s → 1s and 3d → 1s transitions of hydrogenlike atoms. Phys. Rev. A 30, 2441–2448 (1984).
doi: 10.1103/PhysRevA.30.2441
Scheel, S. & Buhmann, S. Y. Macroscopic quantum electrodynamics—concepts and applications. Acta Phys. Slovaca 58, 675–809 (2008).
doi: 10.2478/v10155-010-0092-x
Sibalic, N. et al. ARC: an open-source library for calculating properties of alkali Rydberg atoms. Comput. Phys. Commun. 220, 319–331 (2017).
doi: 10.1016/j.cpc.2017.06.015
Chluba, J. & Sunyaev, R. A. Two-photon transitions in hydrogen and cosmological recombination. Astron. Astrophys. 480, 629–645 (2008).
doi: 10.1051/0004-6361:20077921
Purcell, E. M. Spontaneous emission probabilities at radio frequencies. Phys. Rev. 69, 681–685 (1946).
Guerlin, C. et al. Cavity quantum electrodynamics with a Rydberg-blocked atomic ensemble. Phys. Rev. A 82, 053832 (2010).
doi: 10.1103/PhysRevA.82.053832
Kleppner, D. Inhibited spontaneous emission. Phys. Rev. Lett. 47, 233–236 (1981).
doi: 10.1103/PhysRevLett.47.233
Hulet, R. G., Hilfer, E. S. & Kleppner, D. Inhibited spontaneous emission by a Rydberg atom. Phys. Rev. Lett. 55, 2137–2140 (1985).
doi: 10.1103/PhysRevLett.55.2137
Hunger, D. et al. A fiber Fabry–Perot cavity with high finesse. New J. Phys. 12, 065038 (2010).
doi: 10.1088/1367-2630/12/6/065038
Gallego, J. et al. High-finesse fiber Fabry–Perot cavities: stabilization and mode matching analysis. Appl. Phys. B 122, 47 (2016).
doi: 10.1007/s00340-015-6281-z
Kiilerich, A. H. & Mølmer, K. Input-output theory with quantum pulses. Phys. Rev. Lett. 123, 123604 (2019).
doi: 10.1103/PhysRevLett.123.123604
Sheng, Y. B., Deng, F. G. & Long, G. L. Complete hyperentangled-Bell-state analysis for quantum communication. Phys. Rev. A 82, 032318 (2010).
doi: 10.1103/PhysRevA.82.032318
Hu, X. M. et al. Long-distance entanglement purification for quantum communication. Phys. Rev. Lett. 126, 010503 (2021).
doi: 10.1103/PhysRevLett.126.010503
Cantat-Moltrecht, T. et al. Long-lived circular Rydberg states of laser-cooled rubidium atoms in a cryostat. Phys. Rev. Res. 2, 022032(R) (2020).
doi: 10.1103/PhysRevResearch.2.022032
Hood, C. J., Kimble, H. J. & Ye, J. Characterization of high-finesse mirrors: loss, phase shifts, and mode structure in an optical cavity. Phys. Rev. A 64, 033804 (2001).
doi: 10.1103/PhysRevA.64.033804
Thorpe, M. J. et al. Precise measurements of optical cavity dispersion and mirror coating properties via femtosecond combs. Opt. Express 13, 882–888 (2005).
doi: 10.1364/OPEX.13.000882
Xiang, X. et al. Quantification of nonlocal dispersion cancellation for finite frequency entanglement. Opt. Express 28, 17697–17707 (2020).
doi: 10.1364/OE.390149
Odele, O. D. et al. Tunable delay control of entangled photons based on dispersion cancellation. Opt. Express 23, 21857–21866 (2015).
doi: 10.1364/OE.23.021857

Auteurs

Sutapa Ghosh (S)

Andrew and Erna Viterby Department of Electrical Engineering and Russell Berrie Nanotechnology Institute, Technion-Israel Institute of Technology, Haifa, 32000, Israel. sutapa.g@campus.technion.ac.il.

Nicholas Rivera (N)

Department of Physics, Massachusetts Institute of Technology, Cambridge, MA, USA.

Gadi Eisenstein (G)

Andrew and Erna Viterby Department of Electrical Engineering and Russell Berrie Nanotechnology Institute, Technion-Israel Institute of Technology, Haifa, 32000, Israel.

Ido Kaminer (I)

Andrew and Erna Viterby Department of Electrical Engineering and Russell Berrie Nanotechnology Institute, Technion-Israel Institute of Technology, Haifa, 32000, Israel. kaminer@technion.ac.il.

Classifications MeSH