A Singular Molecule-to-Molecule Transformation on Video: The Bottom-Up Synthesis of Fullerene C

DFT-modeling cyclodehydrogenation fullerene polycyclic aromatic hydrocarbon single-molecule dynamics transmission electron microscopy

Journal

ACS nano
ISSN: 1936-086X
Titre abrégé: ACS Nano
Pays: United States
ID NLM: 101313589

Informations de publication

Date de publication:
24 Aug 2021
Historique:
pubmed: 22 5 2021
medline: 22 5 2021
entrez: 21 5 2021
Statut: ppublish

Résumé

Singular reaction events of small molecules and their dynamics remain a hardly understood territory in chemical sciences since spectroscopy relies on ensemble-averaged data, and microscopic scanning probe techniques show snapshots of frozen scenes. Herein, we report on continuous high-resolution transmission electron microscopic video imaging of the electron-beam-induced bottom-up synthesis of fullerene C

Identifiants

pubmed: 34018713
doi: 10.1021/acsnano.1c02222
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

12804-12814

Auteurs

Dominik Lungerich (D)

Center for Nanomedicine (CNM), Institute for Basic Science (IBS), IBS Hall, 50 Yonsei-ro, Seodaemun-gu, Seoul, 03722, South Korea.
Graduate Program of Nano Biomedical Engineering (NanoBME), Advanced Science Institute, Yonsei University, Seoul, 03722, South Korea.
Department of Chemistry, The University of Tokyo, 7-3-1 Hongo, Bunkyo-ku, Tokyo 113-0033, Japan.

Helen Hoelzel (H)

Department of Chemistry, The University of Tokyo, 7-3-1 Hongo, Bunkyo-ku, Tokyo 113-0033, Japan.
Department of Chemistry and Pharmacy, Organic Chemistry II, Friedrich-Alexander-University Erlangen-Nuernberg (FAU), Nikolaus-Fiebiger-Str. 10, 91058, Erlangen, Germany.

Koji Harano (K)

Department of Chemistry, The University of Tokyo, 7-3-1 Hongo, Bunkyo-ku, Tokyo 113-0033, Japan.

Norbert Jux (N)

Department of Chemistry and Pharmacy, Organic Chemistry II, Friedrich-Alexander-University Erlangen-Nuernberg (FAU), Nikolaus-Fiebiger-Str. 10, 91058, Erlangen, Germany.

Konstantin Yu Amsharov (KY)

Department of Chemistry, Martin-Luther-University Halle-Wittenberg, Kurt-Mothes-Str. 2, 06120 Halle, Germany.

Eiichi Nakamura (E)

Department of Chemistry, The University of Tokyo, 7-3-1 Hongo, Bunkyo-ku, Tokyo 113-0033, Japan.

Classifications MeSH