Laser-induced transient magnons in Sr

iridates time-resolved resonant X-ray scattering transient magnetic excitations

Journal

Proceedings of the National Academy of Sciences of the United States of America
ISSN: 1091-6490
Titre abrégé: Proc Natl Acad Sci U S A
Pays: United States
ID NLM: 7505876

Informations de publication

Date de publication:
01 Jun 2021
Historique:
entrez: 27 5 2021
pubmed: 28 5 2021
medline: 28 5 2021
Statut: ppublish

Résumé

Although ultrafast manipulation of magnetism holds great promise for new physical phenomena and applications, targeting specific states is held back by our limited understanding of how magnetic correlations evolve on ultrafast timescales. Using ultrafast resonant inelastic X-ray scattering we demonstrate that femtosecond laser pulses can excite transient magnons at large wavevectors in gapped antiferromagnets and that they persist for several picoseconds, which is opposite to what is observed in nearly gapless magnets. Our work suggests that materials with isotropic magnetic interactions are preferred to achieve rapid manipulation of magnetism.

Identifiants

pubmed: 34039712
pii: 2103696118
doi: 10.1073/pnas.2103696118
pmc: PMC8179144
pii:
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Déclaration de conflit d'intérêts

The authors declare no competing interest.

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Auteurs

Daniel G Mazzone (DG)

Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory, Upton, NY 11973.
Laboratory for Neutron Scattering and Imaging, Paul Scherrer Institut, CH-5232 Villigen, Switzerland.

Derek Meyers (D)

Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory, Upton, NY 11973.
Department of Physics, Oklahoma State University, Stillwater, OK 74078.

Yue Cao (Y)

Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory, Upton, NY 11973.
Materials Science Division, Argonne National Laboratory, Argonne, IL 60439.

James G Vale (JG)

London Centre for Nanotechnology and Department of Physics and Astronomy, University College London, London WC1E 6BT, United Kingdom.

Cameron D Dashwood (CD)

London Centre for Nanotechnology and Department of Physics and Astronomy, University College London, London WC1E 6BT, United Kingdom.

Youguo Shi (Y)

Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China.

Andrew J A James (AJA)

School of Physical Sciences, The Open University, Milton Keynes MK7 6AA, United Kingdom.

Neil J Robinson (NJ)

Institute for Theoretical Physics, University of Amsterdam, 1098 XH Amsterdam, The Netherlands.

Jiaqi Lin (J)

Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory, Upton, NY 11973.
School of Physical Science and Technology, ShanghaiTech University, Shanghai 201210, China.

Vivek Thampy (V)

Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, Menlo Park, CA 94025.

Yoshikazu Tanaka (Y)

RIKEN SPring-8 Center, Sayo 679-5148, Japan.

Allan S Johnson (AS)

ICFO - The Institute of Photonics Sciences, The Barcelona Institute of Science and Technology, 08860, Castelldefels, Barcelona, Spain.

Hu Miao (H)

Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory, Upton, NY 11973.

Ruitang Wang (R)

School of Physical Science and Technology, ShanghaiTech University, Shanghai 201210, China.

Tadesse A Assefa (TA)

Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory, Upton, NY 11973.

Jungho Kim (J)

Advanced Photon Source, Argonne National Laboratory, Argonne, IL 60439.

Diego Casa (D)

Advanced Photon Source, Argonne National Laboratory, Argonne, IL 60439.

Roman Mankowsky (R)

Max Planck Institute for the Structure and Dynamics of Matter, D-22761 Hamburg, Germany.

Diling Zhu (D)

Linac Coherent Light Source, SLAC National Accelerator Laboratory, Menlo Park, CA 94025.

Roberto Alonso-Mori (R)

Linac Coherent Light Source, SLAC National Accelerator Laboratory, Menlo Park, CA 94025.

Sanghoon Song (S)

Linac Coherent Light Source, SLAC National Accelerator Laboratory, Menlo Park, CA 94025.

Hasan Yavas (H)

Linac Coherent Light Source, SLAC National Accelerator Laboratory, Menlo Park, CA 94025.

Tetsuo Katayama (T)

RIKEN SPring-8 Center, Sayo 679-5148, Japan.

Makina Yabashi (M)

RIKEN SPring-8 Center, Sayo 679-5148, Japan.

Yuya Kubota (Y)

RIKEN SPring-8 Center, Sayo 679-5148, Japan.

Shigeki Owada (S)

RIKEN SPring-8 Center, Sayo 679-5148, Japan.

Jian Liu (J)

Department of Physics and Astronomy, University of Tennessee, Knoxville, TN 37996.

Junji Yang (J)

Department of Physics and Astronomy, University of Tennessee, Knoxville, TN 37996.

Robert M Konik (RM)

Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory, Upton, NY 11973.

Ian K Robinson (IK)

Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory, Upton, NY 11973.
London Centre for Nanotechnology and Department of Physics and Astronomy, University College London, London WC1E 6BT, United Kingdom.

John P Hill (JP)

National Synchrotron Light Source II, Brookhaven National Laboratory, Upton, NY 11973.

Desmond F McMorrow (DF)

London Centre for Nanotechnology and Department of Physics and Astronomy, University College London, London WC1E 6BT, United Kingdom.

Michael Först (M)

Max Planck Institute for the Structure and Dynamics of Matter, D-22761 Hamburg, Germany.

Simon Wall (S)

ICFO - The Institute of Photonics Sciences, The Barcelona Institute of Science and Technology, 08860, Castelldefels, Barcelona, Spain; liuxr@shanghaitech.edu.cn simon.wall@phys.au.dk mdean@bnl.gov.
Department of Physics and Astronomy, Aarhus University, 8000 Aarhus C, Denmark.

Xuerong Liu (X)

School of Physical Science and Technology, ShanghaiTech University, Shanghai 201210, China; liuxr@shanghaitech.edu.cn simon.wall@phys.au.dk mdean@bnl.gov.

Mark P M Dean (MPM)

Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory, Upton, NY 11973; liuxr@shanghaitech.edu.cn simon.wall@phys.au.dk mdean@bnl.gov.

Classifications MeSH