Single-Step Direct Laser Writing of Multimetal Oxygen Evolution Catalysts from Liquid Precursors.

laser writing multimetal catalysis nanostructured materials oxygen evolution reaction transition metal oxides

Journal

ACS nano
ISSN: 1936-086X
Titre abrégé: ACS Nano
Pays: United States
ID NLM: 101313589

Informations de publication

Date de publication:
22 Jun 2021
Historique:
pubmed: 2 6 2021
medline: 2 6 2021
entrez: 1 6 2021
Statut: ppublish

Résumé

We investigate a laser direct-write method to synthesize and deposit metastable, mixed transition metal oxides and evaluate their performance as oxygen evolution reaction catalysts. This laser processing method enabled the rapid synthesis of diverse heterogeneous alloy and oxide catalysts directly from cost-effective solution precursors, including catalysts with a high density of nanocrystalline metal alloy inclusions within an amorphous oxide matrix. The nanoscale heterogeneous structures of the synthesized catalysts were consistent with reactive force-field Monte Carlo calculations. By evaluating the impact of varying transition metal oxide composition ratios, we created a stable Fe

Identifiants

DOI: 10.1021/acsnano.1c00650 PMID: 34061497
pubmed: 34061497
doi: 10.1021/acsnano.1c00650
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

9796-9807

Auteurs

Shannon McGee (S)

Department of Chemistry, The Pennsylvania State University, University Park, Pennsylvania 16802, United States.

Yu Lei (Y)

Department of Physics, The Pennsylvania State University, University Park, Pennsylvania 16802, United States.
Center for Atomically Thin Multifunctional Coatings, The Pennsylvania State University, University Park, Pennsylvania 16802, United States.
Center for 2-Dimensional and Layered Materials, The Pennsylvania State University, University Park, Pennsylvania 16802, United States.

James Goff (J)

Department of Materials Science and Engineering, The Pennsylvania State University, University Park, Pennsylvania 16802, United States.
ORCID: 0000-0001-7026-7200

Collin J Wilkinson (CJ)

Department of Materials Science and Engineering, The Pennsylvania State University, University Park, Pennsylvania 16802, United States.

Nabila Nabi Nova (NN)

Department of Chemistry, The Pennsylvania State University, University Park, Pennsylvania 16802, United States.

Cody Matthew Kindle (CM)

Department of Chemistry, The Pennsylvania State University, University Park, Pennsylvania 16802, United States.

Fu Zhang (F)

Center for Atomically Thin Multifunctional Coatings, The Pennsylvania State University, University Park, Pennsylvania 16802, United States.
Center for 2-Dimensional and Layered Materials, The Pennsylvania State University, University Park, Pennsylvania 16802, United States.
Department of Materials Science and Engineering, The Pennsylvania State University, University Park, Pennsylvania 16802, United States.

Kazunori Fujisawa (K)

Research Initiative for Supra-Materials, Shinshu University, Wakasato 4-17-1, Nagano 380-8553, Japan.

Edgar Dimitrov (E)

Department of Physics, The Pennsylvania State University, University Park, Pennsylvania 16802, United States.
Center for 2-Dimensional and Layered Materials, The Pennsylvania State University, University Park, Pennsylvania 16802, United States.

Susan B Sinnott (SB)

Department of Chemistry, The Pennsylvania State University, University Park, Pennsylvania 16802, United States.
Department of Materials Science and Engineering, The Pennsylvania State University, University Park, Pennsylvania 16802, United States.
Materials Research Institute, The Pennsylvania State University, University Park, Pennsylvania 16802, United States.
Penn State Institutes of Energy and the Environment, The Pennsylvania State University, University Park, Pennsylvania 16802, United States.

Ismaila Dabo (I)

Department of Materials Science and Engineering, The Pennsylvania State University, University Park, Pennsylvania 16802, United States.
Materials Research Institute, The Pennsylvania State University, University Park, Pennsylvania 16802, United States.
Penn State Institutes of Energy and the Environment, The Pennsylvania State University, University Park, Pennsylvania 16802, United States.
ORCID: 0000-0003-0742-030X

Mauricio Terrones (M)

Department of Chemistry, The Pennsylvania State University, University Park, Pennsylvania 16802, United States.
Department of Physics, The Pennsylvania State University, University Park, Pennsylvania 16802, United States.
Center for Atomically Thin Multifunctional Coatings, The Pennsylvania State University, University Park, Pennsylvania 16802, United States.
Center for 2-Dimensional and Layered Materials, The Pennsylvania State University, University Park, Pennsylvania 16802, United States.
Department of Materials Science and Engineering, The Pennsylvania State University, University Park, Pennsylvania 16802, United States.
Research Initiative for Supra-Materials, Shinshu University, Wakasato 4-17-1, Nagano 380-8553, Japan.
ORCID: 0000-0003-0010-2851

Lauren D Zarzar (LD)

Department of Chemistry, The Pennsylvania State University, University Park, Pennsylvania 16802, United States.
Department of Materials Science and Engineering, The Pennsylvania State University, University Park, Pennsylvania 16802, United States.
Materials Research Institute, The Pennsylvania State University, University Park, Pennsylvania 16802, United States.
ORCID: 0000-0002-3287-3602

Classifications MeSH