New insights into correlated materials in the time domain-combining far-infrared excitation with x-ray probes at cryogenic temperatures.
THz excitation
cryogenic
free electron laser
instrumentation
resonant x-ray diffraction
strongly correlated materials
ultrafast
Journal
Journal of physics. Condensed matter : an Institute of Physics journal
ISSN: 1361-648X
Titre abrégé: J Phys Condens Matter
Pays: England
ID NLM: 101165248
Informations de publication
Date de publication:
09 Jul 2021
09 Jul 2021
Historique:
received:
31
01
2021
accepted:
02
06
2021
pubmed:
8
6
2021
medline:
8
6
2021
entrez:
7
6
2021
Statut:
epublish
Résumé
Modern techniques for the investigation of correlated materials in the time domain combine selective excitation in the THz frequency range with selective probing of coupled structural, electronic and magnetic degrees of freedom using x-ray scattering techniques. Cryogenic sample temperatures are commonly required to prevent thermal occupation of the low energy modes and to access relevant material ground states. Here, we present a chamber optimized for high-field THz excitation and (resonant) x-ray diffraction at sample temperatures between 5 and 500 K. Directly connected to the beamline vacuum and featuring both a Beryllium window and an in-vacuum detector, the chamber covers the full (2-12.7) keV energy range of the femtosecond x-ray pulses available at the Bernina endstation of the SwissFEL free electron laser. Successful commissioning experiments made use of the energy tunability to selectively track the dynamics of the structural, magnetic and orbital order of Ca
Identifiants
pubmed: 34098537
doi: 10.1088/1361-648X/ac08b5
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Informations de copyright
Creative Commons Attribution license.