New insights into correlated materials in the time domain-combining far-infrared excitation with x-ray probes at cryogenic temperatures.

THz excitation cryogenic free electron laser instrumentation resonant x-ray diffraction strongly correlated materials ultrafast

Journal

Journal of physics. Condensed matter : an Institute of Physics journal
ISSN: 1361-648X
Titre abrégé: J Phys Condens Matter
Pays: England
ID NLM: 101165248

Informations de publication

Date de publication:
09 Jul 2021
Historique:
received: 31 01 2021
accepted: 02 06 2021
pubmed: 8 6 2021
medline: 8 6 2021
entrez: 7 6 2021
Statut: epublish

Résumé

Modern techniques for the investigation of correlated materials in the time domain combine selective excitation in the THz frequency range with selective probing of coupled structural, electronic and magnetic degrees of freedom using x-ray scattering techniques. Cryogenic sample temperatures are commonly required to prevent thermal occupation of the low energy modes and to access relevant material ground states. Here, we present a chamber optimized for high-field THz excitation and (resonant) x-ray diffraction at sample temperatures between 5 and 500 K. Directly connected to the beamline vacuum and featuring both a Beryllium window and an in-vacuum detector, the chamber covers the full (2-12.7) keV energy range of the femtosecond x-ray pulses available at the Bernina endstation of the SwissFEL free electron laser. Successful commissioning experiments made use of the energy tunability to selectively track the dynamics of the structural, magnetic and orbital order of Ca

Identifiants

pubmed: 34098537
doi: 10.1088/1361-648X/ac08b5
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Informations de copyright

Creative Commons Attribution license.

Auteurs

Roman Mankowsky (R)

Paul Scherrer Institute, Villigen, Switzerland.

Mathias Sander (M)

Paul Scherrer Institute, Villigen, Switzerland.

Serhane Zerdane (S)

European Synchrotron Radiation Facility, Grenoble, France.

Jakub Vonka (J)

Paul Scherrer Institute, Villigen, Switzerland.

Marek Bartkowiak (M)

Paul Scherrer Institute, Villigen, Switzerland.

Yunpei Deng (Y)

Paul Scherrer Institute, Villigen, Switzerland.

Rafael Winkler (R)

Eidgenössische Technische Hochschule Zürich, Zürich, Switzerland.

Flavio Giorgianni (F)

Paul Scherrer Institute, Villigen, Switzerland.

Guy Matmon (G)

Paul Scherrer Institute, Villigen, Switzerland.

Simon Gerber (S)

Paul Scherrer Institute, Villigen, Switzerland.

Paul Beaud (P)

Paul Scherrer Institute, Villigen, Switzerland.

Henrik Till Lemke (HT)

Paul Scherrer Institute, Villigen, Switzerland.

Classifications MeSH