Proton-coupled electron transfer across benzimidazole bridges in bioinspired proton wires.
Journal
Chemical science
ISSN: 2041-6520
Titre abrégé: Chem Sci
Pays: England
ID NLM: 101545951
Informations de publication
Date de publication:
20 Mar 2020
20 Mar 2020
Historique:
entrez:
14
6
2021
pubmed:
20
3
2020
medline:
20
3
2020
Statut:
epublish
Résumé
Designing molecular platforms for controlling proton and electron movement in artificial photosynthetic systems is crucial to efficient catalysis and solar energy conversion. The transfer of both protons and electrons during a reaction is known as proton-coupled electron transfer (PCET) and is used by nature in myriad ways to provide low overpotential pathways for redox reactions and redox leveling, as well as to generate bioenergetic proton currents. Herein, we describe theoretical and electrochemical studies of a series of bioinspired benzimidazole-phenol (BIP) derivatives and a series of dibenzimidazole-phenol (BI
Identifiants
pubmed: 34122850
doi: 10.1039/c9sc06010c
pii: c9sc06010c
pmc: PMC8152432
doi:
Types de publication
Journal Article
Langues
eng
Pagination
3820-3828Informations de copyright
This journal is © The Royal Society of Chemistry.
Déclaration de conflit d'intérêts
There are no conflicts to declare.
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