Swimming droplets in 1D geometries: an active Bretherton problem.


Journal

Soft matter
ISSN: 1744-6848
Titre abrégé: Soft Matter
Pays: England
ID NLM: 101295070

Informations de publication

Date de publication:
14 Jul 2021
Historique:
pubmed: 22 6 2021
medline: 22 6 2021
entrez: 21 6 2021
Statut: ppublish

Résumé

We investigate experimentally the behavior of self-propelled water-in-oil droplets, confined in capillaries of different square and circular cross-sections. The droplet's activity comes from the formation of swollen micelles at its interface. In straight capillaries the velocity of the droplet decreases with increasing confinement. However, at very high confinement, the velocity converges toward a non-zero value, so that even very long droplets swim. Stretched circular capillaries are used to explore even higher confinement. The lubrication layer around the droplet then takes a non-uniform thickness which constitutes a significant difference to usual flow-driven passive droplets. A neck forms at the rear of the droplet, deepens with increasing confinement, and eventually undergoes successive spontaneous splitting events for large enough confinement. Such observations stress the critical role of the activity of the droplet interface in the droplet's behavior under confinement. We then propose an analytical formulation by integrating the interface activity and the swollen micelle transport problem into the classical Bretherton approach. The model accounts for the convergence of the droplet's velocity to a finite value for large confinement, and for the non-classical shape of the lubrication layer. We further discuss on the saturation of the micelle concentration along the interface, which would explain the divergence of the lubrication layer thickness for long enough droplets, eventually leading to spontaneous droplet division.

Identifiants

pubmed: 34152345
doi: 10.1039/d1sm00387a
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

6646-6660

Auteurs

Charlotte de Blois (C)

UMR CNRS Gulliver 7083, ESPCI Paris, PSL Research University, 75005 Paris, France. Charlotte.de-blois@espci.fr Mathilde.Reyssat@espci.fr and Okinawa Institute of Science and Technology Graduate University, Onna-son, Okinawa 904-0495, Japan.

Vincent Bertin (V)

UMR CNRS Gulliver 7083, ESPCI Paris, PSL Research University, 75005 Paris, France. Charlotte.de-blois@espci.fr Mathilde.Reyssat@espci.fr and Univ. Bordeaux, CNRS, LOMA, UMR 5798, 33405 Talence, France.

Saori Suda (S)

Department of Physics, Graduate School of Science, Kyoto University, Kitashirakawa-Oiwakecho, Sakyo-ku, Kyoto 606-8502, Japan.

Masatoshi Ichikawa (M)

Department of Physics, Graduate School of Science, Kyoto University, Kitashirakawa-Oiwakecho, Sakyo-ku, Kyoto 606-8502, Japan.

Mathilde Reyssat (M)

UMR CNRS Gulliver 7083, ESPCI Paris, PSL Research University, 75005 Paris, France. Charlotte.de-blois@espci.fr Mathilde.Reyssat@espci.fr.

Olivier Dauchot (O)

UMR CNRS Gulliver 7083, ESPCI Paris, PSL Research University, 75005 Paris, France. Charlotte.de-blois@espci.fr Mathilde.Reyssat@espci.fr.

Classifications MeSH