Lanthanide (Ce, Nd, Eu) environments and leaching behavior in borosilicate glasses.
Journal
Scientific reports
ISSN: 2045-2322
Titre abrégé: Sci Rep
Pays: England
ID NLM: 101563288
Informations de publication
Date de publication:
24 Jun 2021
24 Jun 2021
Historique:
received:
08
02
2021
accepted:
10
06
2021
entrez:
25
6
2021
pubmed:
26
6
2021
medline:
26
6
2021
Statut:
epublish
Résumé
Borosilicate glasses will be used to stabilize the high-level radioactive wastes for disposal in a geological repository. Understanding the effects of actinide addition to a borosilicate glass matrix is of great importance in view of waste immobilization. Lanthanides were considered as chemical surrogates for actinides. The local structures of Ce
Identifiants
pubmed: 34168262
doi: 10.1038/s41598-021-92777-w
pii: 10.1038/s41598-021-92777-w
pmc: PMC8225880
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
13272Références
Veliscel-Carolan, J. Separation of actinides from spent nuclear fuel: A review. J. Haz. Mat. 318, 266–281 (2016).
doi: 10.1016/j.jhazmat.2016.07.027
Chun, K. S., Kim, S. S. & Kang, C. H. Release of boron and cesium or uranium from simulated borosilicate waste glasses through a compacted Ca-bentonite layer. J. Nucl. Mat. 298, 150–154 (2001).
doi: 10.1016/S0022-3115(01)00612-2
Jantzen, C. M., Brown, K. G. & Pickett, J. B. Impact of phase separation on durability in phosphate containing borosilicate waste glasses for INEEL. WSRC-MS-2000–00307 (Westinghouse Savannah River Company Report, 2000).
Stefanovsky, S. V., Shiryaev, A. A., Zubavitchus, J. V., Veligjanin, A. A. & Marra, J. C. Valence state and speciation of uranium ions in borosilicate glasses with a high iron and aluminum content. Glass Phys. Chem. 35, 141–148 (2009).
doi: 10.1134/S1087659609020035
Lopez, C. et al. Solubility of actinide surrogates in nuclear glasses. J. Nucl. Mater 312, 76–80 (2003).
doi: 10.1016/S0022-3115(02)01549-0
Loiseau, P., Caurant, D., Baffier, N., Mazerolles, L. & Fillet, C. Glass-ceramic nuclear waste forms obtained from SiO
doi: 10.1016/j.jnucmat.2004.05.020
Shannon, R. D. Revised effective ionic radii and systematic studies of interatomic distances in halides and chalcogenides. Acta Cryst. Sect. A 32, 751–767 (1976).
doi: 10.1107/S0567739476001551
Fabian, M., Svab, E., Proffen, Th. & Veress, E. Structure study of multi-component borosilicate glasses from high-Q neutron diffraction measurement and RMC modelling. J. Non-Cryst. Solids 354, 3299–3307 (2008).
doi: 10.1016/j.jnoncrysol.2008.01.024
Fabian, M. et al. Structural investigation of borosilicate glasses containing lanthanide ions. Sci. Rep. 10, 7835 (2020).
pubmed: 32398655
pmcid: 7217859
doi: 10.1038/s41598-020-64754-2
Waasmaier, D. & Kirfel, A. New analytical scattering-factor functions for free atoms and ions. Acta Crystallogr. A 51, 416–451 (1995).
doi: 10.1107/S0108767394013292
Fabian, M. et al. Network structure of 0.7SiO
Svab, E., Fabian, M., Veress, E. & Proffen, Th. Short- and intermediate range order in borosilicate waste glasses. Acta Cryst. A63, s58–s59 (2007).
doi: 10.1107/S0108767307098728
Du, L.-S. & Stebbins, J. F. Solid-state NMR study of metastable immiscibility in alkali borosilicate glasses. J. Non-Cryst. Solids 315, 239–255 (2003).
doi: 10.1016/S0022-3093(02)01604-6
Bajaj, A., Khanna, A., Chen, B. & Longstaffe, J. G. Structural investigation of bismuth borate glasses and crystalline phases. J. Non-Cryst. Solids 355, 45–53 (2009).
doi: 10.1016/j.jnoncrysol.2008.09.033
Gou, F., Greaves, G. N., Smith, W. & Winter, R. Molecular dynamics simulation of sodium borosilicate glasses. J. Non-Cryst. Solids 293–295, 539–546 (2001).
doi: 10.1016/S0022-3093(01)00775-X
Sato, T. et al. Network structure of borate and germinate glasses studied by means of pulsed neutron scattering. J. Non-Cryst. Solids 232, 574–580 (1998).
doi: 10.1016/S0022-3093(98)00525-0
Ohtori, N. et al. Short-range structure of alkaline-earth borate glasses by poulsed neutron diffraction and molecular dynamic simulation. J. Non-Cryst. Solids 293–295, 136–145 (2001).
doi: 10.1016/S0022-3093(01)00662-7
Qian, M., Li, H., Li, L. & Strachan, D. M. Extended electron energy loss fine structure simulation of the local boron environment in sodium aluminoborosilicate glasses containing gadolinium. J. Non-Cryst. Solids 328, 90–101 (2003).
doi: 10.1016/S0022-3093(03)00477-0
Burns, A. E. et al. Structure of binary neodymium borate glasses by infrared spectroscopy. J. Non-Cryst. Solids 352, 2364–2366 (2006).
doi: 10.1016/j.jnoncrysol.2006.03.043
El-Damrawi, G., Gharghar, F. & Ramadan, R. More insight on structure of new binary cerium borate glasses. New J. Glass Ceram. 8, 12–21 (2018).
doi: 10.4236/njgc.2018.81002
Fabian, M. & Araczki, C. Basic network structure of SiO
doi: 10.1088/0031-8949/91/5/054004
Jollivet, P., Lopez, C., Auwer, C. D. & Simoni, E. Evolution of local environment of cerium and neodymium during simplified SON68 glass alteration. J. Nucl. Mat. 346, 253–265 (2005).
doi: 10.1016/j.jnucmat.2005.06.017
Du, J. et al. Structure of cerium phosphate glasses: Molecular dynamics simulation. J. Am. Ceram. Soc. 94(8), 2393–2401 (2011).
doi: 10.1111/j.1551-2916.2011.04514.x
Majerus, O., Tregouet, H., Caurant, D. & Pytalev, D. Comparative study of the rare earth environment in rare earth metaborate glasses (REB
doi: 10.1016/j.jnoncrysol.2015.05.031
Bouty, O., Delaye, J. M. & Peuget, S. Europium structural effect on a borosilicate glass of nuclear interest. Proc. Chem. 7, 540–547 (2012).
doi: 10.1016/j.proche.2012.10.082
Kokou, L. & Du, J. Rare earth ion clustering behavior in europium doped silicate glasses: Simulation size and glass structure effect. J. Non-Cryst. Solids 358, 3408–3417 (2012).
doi: 10.1016/j.jnoncrysol.2012.01.068
Zhu, H., Wang, F., Liao, Q., Wang, Y. & Zhu, Y. Effect of CeO
doi: 10.1016/j.matchemphys.2020.122936
Cicconi, M. R. et al. Europium oxidation state and local structure in silicate glasses. Am. Mineral 97, 918–929 (2012).
doi: 10.2138/am.2012.4041
Müller-Bunz, H., Nikelski, T. & Schleid, T. Single crystals of the neodymium(III) meta-borate Nd(BO
doi: 10.1515/znb-2003-0503
Tas, A. C. & Akinc, M. Crystal structures of the high-temperature forms of Ln2Si2O7 (Ln=La, Ce, Pr, Nd, Sm) revisited. J. Am. Ceram. Soc. 77, 2968–2970 (1994).
doi: 10.1111/j.1151-2916.1994.tb04532.x
Li, H. et al. Neodymium (III) in alumino-borosilicate glasses. J. Non-Cryst. Solids 278, 35–57 (2000).
doi: 10.1016/S0022-3093(00)00327-6
Sen, S. Atomic environment of high-field strength Nd and Al cations as dopants and major components in silicate glasses: Nd L
doi: 10.1016/S0022-3093(99)00564-5
Quartieri, S. et al. Characterization of trace Nd and Ce site preference and coordination in natural melanites: A combined X-ray diffraction and high-energy XAFS study. Phys. Chem. Minerals 29, 495–502 (2002).
doi: 10.1007/s00269-002-0251-9
Yamaguchi, H. & Takebe, H. Local structure of rare-earth ions in alkali silicate glasses studied by extended X-ray absorption fine structure. Jpn. J. Appl. Phys. 38, 168–171 (1999).
doi: 10.7567/JJAPS.38S1.168
Ysker, J. S. & Hoffmann, W. Die Kristallstructur des La[B
doi: 10.1007/BF00600055
Persson, K. Materials Data on Eu
Estelle, M. et al. Investigation of local environment around rare earth (La and Eu) by fluorescence line narrowing during borosilicate glass alteration. J. Lum. 145, 213–218 (2014).
doi: 10.1016/j.jlumin.2013.07.051
Inoue, H. et al. An XAFS study of the local structure of Eu
doi: 10.2109/jcersj2.20043
ASTM C-1285–02, Standard test methods for determining chemical durability of nuclear, hazardous and mixed waste glasses and multiphase glass ceramics: the product consistency test (PCT), ASTM International, 100 Barr Harbor Drive, PO Box C700, West Conshohocken, PA 19428–2959, United States.
ASTM C-1285–21, Standard test methods for determining chemical durability of nuclear, hazardous, and mixed waste glasses and multiphase glass ceramics: the product consistency test (PCT), ASTM International, 100 Barr Harbor Drive, PO Box C700, West Conshohocken, PA 19428–2959, United States.
Wu, K. et al. Synthesis of pyrochlore-borosilicate glass-ceramics for immobilization of high-level nuclear waste. Ceram. Int. 46, 6085–6094 (2020).
doi: 10.1016/j.ceramint.2019.11.071
Maeda, T., Ohmori, H., Mitsui, S. & Banba, T. Corrosion behavior of simulated HLW glass in the presence of magnesium ion. Int. J. Corros. 2011, 1–6 (2011).
doi: 10.1155/2011/796457
Kim, M. & Heo, J. Calcium-borosilicate glass-ceramics wasteforms to immobilize rare-earth oxide wastes from pyro-processing. J. Nucl. Mater. 467, 224–228 (2015).
doi: 10.1016/j.jnucmat.2015.09.040
Roberts, N., Porter, P., Brow, R. K. Phase separation and crystallization of complex borosilicate melts for glass-ceramic waste forms, Missouri University of Science and Technology, Project No. 15–8112, DE-NE0008411 (2018).
Zhu, H., Wang, F., Liao, Q. & Zhu, Y. Synthesis and characterization of zirconolite-sodium borosilicate glass-ceramics for nuclear waste immobilization. J. Nucl. Mater. 532, 152026 (2020).
doi: 10.1016/j.jnucmat.2020.152026
U.S. Department of Energy (DOE), Design, Construction, and Commissioning of the Hanford Tank Waste Treatment and Immobilization Plant, DOE Office of River Protection, Richland, WA; Contract with Bechtel National, Inc., San Francisco, CA, Contract No.: DE-AC27–01RV14136 (2001).
Ojovan, N. V. et al. Product consistency test of fully radioactive high-sodium content borosilicate glass K-26. Mat. Res. Soc. Symp. Proc. 824, 1–6 (2004).
doi: 10.1557/PROC-824-CC8.14
Estelle, M. et al. Chemical durability of lanthanum-enriched borosilicate glass. Int. J. Appl. Glass Sci. 4, 383–394 (2013).
doi: 10.1111/ijag.12054
Backhouse, D. J. et al. Corrosion of the international simple glass under acidic to hyperalkaline conditions. Mat. Degrad. 29, 10 (2018).
Miekina, M. Crystal formation during the vitrification of HLW in Ca/Zn base glass., PhD thesis, University of Sheffield pp. 92 (2018).
Vance, E. R. et al. The influence of ZnO incoporation on the aqueous leaching characteristics if a borosilicate glass. J. Nucl. Mat. 494, 37–45 (2017).
doi: 10.1016/j.jnucmat.2017.06.035
Schell, N. et al. The high energy materials science beamline (HEMS) at PETRA III. Mat. Sci. Forum 772, 57–61 (2013).
doi: 10.4028/www.scientific.net/MSF.772.57
Juhás, P., Davis, T., Farrow, C. L. & Billinge, S. J. L. PDFgetX3: A rapid and highly automatable program for processing powder diffraction data into total scattering pair distribution functions. J. Appl. Cryst. 46, 560–566 (2013).
doi: 10.1107/S0021889813005190
Gereben, O., Jovari, P., Temleitner, L. & Pusztai, L. A new version of the RMC
Cicco, A. D. et al. Novel XAFS capabilities at Elettra synchrotron light source. J. Phys. Conf. Series 190, 012043 (2009).
doi: 10.1088/1742-6596/190/1/012043
Farrel Lytle database. (Accessed 21 Jan 2021); http://ixs.iit.edu/database/data/Farrel_Lytle_data/RAW/Ce/index.html .
XAS Data Library. (Accessed 11 May 2021); https://github.com/XraySpectroscopy/XASDataLibrary .
Ravel, B. & Newville, M. ATHENA, ARTEMIS, HEPHAESTUS: Data analysis for X-ray absorption spectroscopy using IFEFFIT. J. Sync. Rad. 12, 537–541 (2005).
doi: 10.1107/S0909049505012719
Ankudinov, A. L., Bouldin, C., Rehr, J. J., Sims, J. & Hung, H. Parallel calculation of electron multiple scattering using Lanczos algorithms. Phys. Rev. B 65, 104107 (2002).
doi: 10.1103/PhysRevB.65.104107
Newville, M. EXAFS analysis using FEFF and FEFFIT. J. Synch. Rad. 8, 96–100 (2001).
doi: 10.1107/S0909049500016290
Poinssot, C. & Gin, S. Long-term behavior science: The cornerstone approach for reliably assessing the long-term performance of nuclear waste. J. Nuc. Mat. 420, 182–192 (2012).
doi: 10.1016/j.jnucmat.2011.09.012
Vienna, J. D., Ryan, J. V., Gin, S. & Inagaki, Y. Current understanding and remaining challenges in modeling long-term degradation of borosilicate nuclear waste glasses. Int. J. Appl. Glass Sci 4, 283–294 (2013).
doi: 10.1111/ijag.12050