Polaron Masses in CH_{3}NH_{3}PbX_{3} Perovskites Determined by Landau Level Spectroscopy in Low Magnetic Fields.
Journal
Physical review letters
ISSN: 1079-7114
Titre abrégé: Phys Rev Lett
Pays: United States
ID NLM: 0401141
Informations de publication
Date de publication:
11 Jun 2021
11 Jun 2021
Historique:
received:
05
07
2020
revised:
14
03
2021
accepted:
11
05
2021
entrez:
25
6
2021
pubmed:
26
6
2021
medline:
26
6
2021
Statut:
ppublish
Résumé
We investigate the electron-phonon coupling in CH_{3}NH_{3}PbX_{3} lead halide perovskites through the observation of Landau levels and high-order excitons at weak magnetic fields, where the cyclotron energy is significantly smaller than the longitudinal optical phonon energy. The reduced masses of the carriers and the exciton binding energies obtained from these data are clearly influenced by polaron formation. We analyze the field-dependent polaronic and excitonic properties, and show that they can be quantitatively reproduced by the Fröhlich large polaron model.
Identifiants
pubmed: 34170157
doi: 10.1103/PhysRevLett.126.237401
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM