Polaron Masses in CH_{3}NH_{3}PbX_{3} Perovskites Determined by Landau Level Spectroscopy in Low Magnetic Fields.


Journal

Physical review letters
ISSN: 1079-7114
Titre abrégé: Phys Rev Lett
Pays: United States
ID NLM: 0401141

Informations de publication

Date de publication:
11 Jun 2021
Historique:
received: 05 07 2020
revised: 14 03 2021
accepted: 11 05 2021
entrez: 25 6 2021
pubmed: 26 6 2021
medline: 26 6 2021
Statut: ppublish

Résumé

We investigate the electron-phonon coupling in CH_{3}NH_{3}PbX_{3} lead halide perovskites through the observation of Landau levels and high-order excitons at weak magnetic fields, where the cyclotron energy is significantly smaller than the longitudinal optical phonon energy. The reduced masses of the carriers and the exciton binding energies obtained from these data are clearly influenced by polaron formation. We analyze the field-dependent polaronic and excitonic properties, and show that they can be quantitatively reproduced by the Fröhlich large polaron model.

Identifiants

pubmed: 34170157
doi: 10.1103/PhysRevLett.126.237401
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

237401

Auteurs

Yasuhiro Yamada (Y)

Graduate School of Science, Chiba University, Inage, Chiba 263-8522, Japan.

Hirofumi Mino (H)

Graduate School of Global and Transdisciplinary Studies, Chiba University, Inage, Chiba 263-8522, Japan.

Takuya Kawahara (T)

Graduate School of Education, Chiba University, Inage, Chiba 263-8522, Japan.

Kenichi Oto (K)

Graduate School of Science, Chiba University, Inage, Chiba 263-8522, Japan.

Hidekatsu Suzuura (H)

Graduate School of Engineering, Hokkaido University, Sapporo 060-8628, Japan.

Yoshihiko Kanemitsu (Y)

Institute for Chemical Research, Kyoto University, Uji, Kyoto 611-0011, Japan.

Classifications MeSH