Cathelicidin and PMB neutralize endotoxins by multifactorial mechanisms including LPS interaction and targeting of host cell membranes.


Journal

Proceedings of the National Academy of Sciences of the United States of America
ISSN: 1091-6490
Titre abrégé: Proc Natl Acad Sci U S A
Pays: United States
ID NLM: 7505876

Informations de publication

Date de publication:
06 07 2021
Historique:
entrez: 29 6 2021
pubmed: 30 6 2021
medline: 15 12 2021
Statut: ppublish

Résumé

Antimicrobial peptides (AMPs) contribute to an effective protection against infections. The antibacterial function of AMPs depends on their interactions with microbial membranes and lipids, such as lipopolysaccharide (LPS; endotoxin). Hyperinflammation induced by endotoxin is a key factor in bacterial sepsis and many other human diseases. Here, we provide a comprehensive profile of peptide-mediated LPS neutralization by systematic analysis of the effects of a set of AMPs and the peptide antibiotic polymyxin B (PMB) on the physicochemistry of endotoxin, macrophage activation, and lethality in mice. Mechanistic studies revealed that the host defense peptide LL-32 and PMB each reduce LPS-mediated activation also via a direct interaction of the peptides with the host cell. As a biophysical basis, we demonstrate modifications of the structure of cholesterol-rich membrane domains and the association of glycosylphosphatidylinositol (GPI)-anchored proteins. Our discovery of a host cell-directed mechanism of immune control contributes an important aspect in the development and therapeutic use of AMPs.

Identifiants

pubmed: 34183393
pii: 2101721118
doi: 10.1073/pnas.2101721118
pmc: PMC8271772
pii:
doi:

Substances chimiques

Antimicrobial Cationic Peptides 0
Cathelicidins 0
Lipopolysaccharides 0
Cholesterol 97C5T2UQ7J
Polymyxin B J2VZ07J96K

Types de publication

Journal Article Research Support, Non-U.S. Gov't

Langues

eng

Sous-ensembles de citation

IM

Déclaration de conflit d'intérêts

Competing interest statement: K.B. holds a patent for Aspidasept® and is the Chief Executive Officer of Brandenburg Antiinfectiva GmbH.

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Auteurs

Andra B Schromm (AB)

Division of Immunobiophysics, Research Center Borstel, Leibniz Lung Center, D-23845 Borstel, Germany; aschromm@fz-borstel.de.

Laura Paulowski (L)

Division of Immunobiophysics, Research Center Borstel, Leibniz Lung Center, D-23845 Borstel, Germany.
Division of Biophysics, Research Center Borstel, Leibniz Lung Center, D-23845 Borstel, Germany.

Yani Kaconis (Y)

Division of Biophysics, Research Center Borstel, Leibniz Lung Center, D-23845 Borstel, Germany.

Franziska Kopp (F)

Division of Immunobiophysics, Research Center Borstel, Leibniz Lung Center, D-23845 Borstel, Germany.
Division of Biophysics, Research Center Borstel, Leibniz Lung Center, D-23845 Borstel, Germany.

Max Koistinen (M)

Division of Biophysics, Research Center Borstel, Leibniz Lung Center, D-23845 Borstel, Germany.

Annemarie Donoghue (A)

Division of Biophysics, Research Center Borstel, Leibniz Lung Center, D-23845 Borstel, Germany.

Susanne Keese (S)

Division of Immunobiophysics, Research Center Borstel, Leibniz Lung Center, D-23845 Borstel, Germany.

Christian Nehls (C)

Division of Biophysics, Research Center Borstel, Leibniz Lung Center, D-23845 Borstel, Germany.

Julia Wernecke (J)

Division of Biophysics, Research Center Borstel, Leibniz Lung Center, D-23845 Borstel, Germany.
Deutsches Elektronen-Synchrotron, D-22607 Hamburg, Germany.

Patrick Garidel (P)

Biophysikalische Chemie, Martin-Luther-Universität Halle-Wittenberg, D-06108 Halle, Germany.

Eva Sevcsik (E)

Institute of Applied Physics at TU Wien, Vienna 1040, Austria.

Karl Lohner (K)

Institute of Molecular Biosciences, Biophysics Division, University of Graz, A-8010 Graz, Austria.
BioTechMed-Graz, A-8010 Graz, Austria.

Susana Sanchez-Gomez (S)

Department of Microbiology and Parasitology, University of Navarra, E-31008 Pamplona, Spain.

Guillermo Martinez-de-Tejada (G)

Department of Microbiology and Parasitology, University of Navarra, E-31008 Pamplona, Spain.
Navarra Institute for Health Research, E-31008 Pamplona, Spain.

Klaus Brandenburg (K)

Division of Biophysics, Research Center Borstel, Leibniz Lung Center, D-23845 Borstel, Germany.

Mario Brameshuber (M)

Institute of Applied Physics at TU Wien, Vienna 1040, Austria.

Gerhard J Schütz (GJ)

Institute of Applied Physics at TU Wien, Vienna 1040, Austria.

Jörg Andrä (J)

Division of Biophysics, Research Center Borstel, Leibniz Lung Center, D-23845 Borstel, Germany.
Department of Biotechnology, Faculty of Life Sciences, Hamburg University of Applied Sciences, D-21033 Hamburg, Germany.

Thomas Gutsmann (T)

Division of Biophysics, Research Center Borstel, Leibniz Lung Center, D-23845 Borstel, Germany.

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Classifications MeSH