Supramolecular Assembly of Conjugated Polymers under Vibrational Strong Coupling.
assembly
kinetics
strong coupling
supramolecular
vibrations
Journal
Angewandte Chemie (International ed. in English)
ISSN: 1521-3773
Titre abrégé: Angew Chem Int Ed Engl
Pays: Germany
ID NLM: 0370543
Informations de publication
Date de publication:
01 Sep 2021
01 Sep 2021
Historique:
revised:
04
06
2021
received:
29
04
2021
pubmed:
14
7
2021
medline:
14
7
2021
entrez:
13
7
2021
Statut:
ppublish
Résumé
Strong coupling plays a significant role in influencing chemical reactions and tuning material properties by modifying the energy landscapes of the systems. Here we study the effect of vibrational strong coupling (VSC) on supramolecular organization. For this purpose, a rigid-rod conjugated polymer known to form gels was strongly coupled together with its solvent in a microfluidic IR Fabry-Perot cavity. Absorption and fluorescence studies indicate a large modification of the self-assembly under such cooperative VSC. Electron microscopy confirms that in this case, the supramolecular morphology is totally different from that observed in the absence of strong coupling. In addition, the self-assembly kinetics are altered and depend on the solvent vibration under VSC. The results are compared to kinetic isotope effects on the self-assembly to help clarify the role of different parameters under strong coupling. These findings indicate that VSC is a valuable new tool for controlling supramolecular assemblies with broad implications for the molecular and material sciences.
Identifiants
pubmed: 34255910
doi: 10.1002/anie.202105840
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
19665-19670Subventions
Organisme : Agence Nationale de la Recherche
ID : ANR-10-EQPX-52-01
Organisme : Agence Nationale de la Recherche
ID : ANR-10-LABX- 0026 CSC
Organisme : Agence Nationale de la Recherche
ID : ANR-10-IDEX-0002-02
Organisme : H2020 Marie Skłodowska-Curie Actions
ID : 811284
Organisme : Japan Society for the Promotion of Science
ID : JP20J00845
Organisme : H2020 European Research Council
ID : 788482
Informations de copyright
© 2021 Wiley-VCH GmbH.
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