Understanding polyoxometalates as water oxidation catalysts through iron


Journal

Chemical science
ISSN: 2041-6520
Titre abrégé: Chem Sci
Pays: England
ID NLM: 101545951

Informations de publication

Date de publication:
01 Jul 2021
Historique:
received: 20 02 2021
accepted: 13 05 2021
entrez: 14 7 2021
pubmed: 15 7 2021
medline: 15 7 2021
Statut: epublish

Résumé

Cobalt polyoxometalates (Co-POMs) have emerged as promising water oxidation catalysts (WOCs), with the added advantage of their molecular nature despite being metal oxide fragments. In comparison with metal oxides, that do not offer well-defined active surfaces, POMs have a controlled, discrete structure that allows for precise correlations between experiment and computational analyses. Thus, beyond highly active WOCs, POMs are also model systems to gain deeper mechanistic understanding on the oxygen evolution reaction (OER). The tetracobalt Weakley sandwich [Co

Identifiants

pubmed: 34257875
doi: 10.1039/d1sc01016f
pii: d1sc01016f
pmc: PMC8246111
doi:

Types de publication

Journal Article

Langues

eng

Pagination

8755-8766

Informations de copyright

This journal is © The Royal Society of Chemistry.

Déclaration de conflit d'intérêts

There are no conflicts to declare.

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Auteurs

Khalid Azmani (K)

Institute of Chemical Research of Catalonia (ICIQ), The Barcelona Institute of Science and Technology (BIST) Av. Països Catalans, 16 Tarragona E-43007 Spain.
Departament de Química Física i Inorgànica, Universitat Rovira i Virgili Marcel·lí Domingo 1 E-43007 Tarragona Spain maria.besora@urv.cat josepmaria.poblet@urv.cat.

Maria Besora (M)

Departament de Química Física i Inorgànica, Universitat Rovira i Virgili Marcel·lí Domingo 1 E-43007 Tarragona Spain maria.besora@urv.cat josepmaria.poblet@urv.cat.

Joaquín Soriano-López (J)

School of Chemistry & AMBER Center, Trinity College, University of Dublin Dublin D02 PN40 Ireland sorianoj@tcd.ie.

Meriem Landolsi (M)

Departament de Química Física i Inorgànica, Universitat Rovira i Virgili Marcel·lí Domingo 1 E-43007 Tarragona Spain maria.besora@urv.cat josepmaria.poblet@urv.cat.

Anne-Lucie Teillout (AL)

Equipe d'Electrochimie et de Photo-électrochimie, Institut de Chimie Physique, UMR 8000, CNRS, Université Paris Saclay Orsay F-91405 France.

Pedro de Oliveira (P)

Equipe d'Electrochimie et de Photo-électrochimie, Institut de Chimie Physique, UMR 8000, CNRS, Université Paris Saclay Orsay F-91405 France.

Israël-Martyr Mbomekallé (IM)

Equipe d'Electrochimie et de Photo-électrochimie, Institut de Chimie Physique, UMR 8000, CNRS, Université Paris Saclay Orsay F-91405 France.

Josep M Poblet (JM)

Departament de Química Física i Inorgànica, Universitat Rovira i Virgili Marcel·lí Domingo 1 E-43007 Tarragona Spain maria.besora@urv.cat josepmaria.poblet@urv.cat.

José-Ramón Galán-Mascarós (JR)

Institute of Chemical Research of Catalonia (ICIQ), The Barcelona Institute of Science and Technology (BIST) Av. Països Catalans, 16 Tarragona E-43007 Spain.
ICREA, Pg. Lluís Companys 23 08010 Barcelona Spain.

Classifications MeSH